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| Hauptseite > Publikationsdatenbank > Towards bio-upcycling of polyethylene terephthalate > print |
| 001 | 892391 | ||
| 005 | 20210902140218.0 | ||
| 024 | 7 | _ | |a 10.1016/j.ymben.2021.03.011 |2 doi |
| 024 | 7 | _ | |a 1096-7176 |2 ISSN |
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| 082 | _ | _ | |a 610 |
| 100 | 1 | _ | |a Tiso, Till |0 0000-0003-4420-5609 |b 0 |
| 245 | _ | _ | |a Towards bio-upcycling of polyethylene terephthalate |
| 260 | _ | _ | |a Orlando, Fla. |c 2021 |b Academic Press |
| 336 | 7 | _ | |a article |2 DRIVER |
| 336 | 7 | _ | |a Output Types/Journal article |2 DataCite |
| 336 | 7 | _ | |a Journal Article |b journal |m journal |0 PUB:(DE-HGF)16 |s 1630575340_18928 |2 PUB:(DE-HGF) |
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| 500 | _ | _ | |a Biotechnologie 1 |
| 520 | _ | _ | |a Over 359 million tons of plastics were produced worldwide in 2018, with significant growth expected in the near future, resulting in the global challenge of end-of-life management. The recent identification of enzymes that degrade plastics previously considered non-biodegradable opens up opportunities to steer the plastic recycling industry into the realm of biotechnology.Here, the sequential conversion of post-consumer polyethylene terephthalate (PET) into two types of bioplastics is presented: a medium chain-length polyhydroxyalkanoate (PHA) and a novel bio-based poly(amide urethane) (bio-PU). PET films are hydrolyzed by a thermostable polyester hydrolase yielding highly pure terephthalate and ethylene glycol. The obtained hydrolysate is used directly as a feedstock for a terephthalate-degrading Pseudomonas umsongensis GO16, also evolved to efficiently metabolize ethylene glycol, to produce PHA. The strain is further modified to secrete hydroxyalkanoyloxy-alkanoates (HAAs), which are used as monomers for the chemo-catalytic synthesis of bio-PU. In short, a novel value-chain for PET upcycling is shown that circumvents the costly purification of PET monomers, adding technological flexibility to the global challenge of end-of-life management of plastics. |
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| 700 | 1 | _ | |a Narancic, Tanja |0 P:(DE-HGF)0 |b 1 |
| 700 | 1 | _ | |a Wei, Ren |0 0000-0003-3876-1350 |b 2 |
| 700 | 1 | _ | |a Pollet, Eric |0 0000-0002-4920-7024 |b 3 |
| 700 | 1 | _ | |a Beagan, Niall |0 P:(DE-HGF)0 |b 4 |
| 700 | 1 | _ | |a Schröder, Katja |0 P:(DE-HGF)0 |b 5 |
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| 700 | 1 | _ | |a Avérous, Luc |0 P:(DE-HGF)0 |b 11 |
| 700 | 1 | _ | |a Zimmermann, Wolfgang |0 0000-0002-5730-6663 |b 12 |
| 700 | 1 | _ | |a O'Connor, Kevin |0 P:(DE-HGF)0 |b 13 |
| 700 | 1 | _ | |a Blank, Lars M. |0 0000-0003-0961-4976 |b 14 |e Corresponding author |
| 773 | _ | _ | |a 10.1016/j.ymben.2021.03.011 |g Vol. 66, p. 167 - 178 |0 PERI:(DE-600)1471017-1 |p 167 - 178 |t Metabolic engineering |v 66 |y 2021 |x 1096-7176 |
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