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@ARTICLE{Guo:892554,
author = {Guo, H. and Ritter, C. and Su, Y. and Komarek, A. C. and
Gardner, J. S.},
title = {{D}istinct magnetic ground states of {R}2{Z}n{I}r{O}6 ( {R}
= {L}a , {N}d ) determined by neutron powder diffraction},
journal = {Physical review / B},
volume = {103},
number = {6},
issn = {2469-9969},
address = {Woodbury, NY},
publisher = {Inst.},
reportid = {FZJ-2021-02153},
pages = {L060402},
year = {2021},
abstract = {Double-perovskite iridates A2ZnIrO6 (A=alkaline or
lanthanide) show complex magnetic behaviors ranging from
weak ferromagnetism to successive antiferromagnetic
transitions. Here we report the static (dc) and dynamic (ac)
magnetic susceptibility and neutron powder diffraction
measurements for A=La and Nd compounds to elucidate the
magnetic ground state. Below 10 K, the A=La compound is best
described as canted iridium moments in an antiferromagnet
arrangement with a propagation vector k = 0 and a net
ferromagnetic component along the c axis. On the other hand,
Nd2ZnIrO6 is described well as an antiferromagnet with a
propagation vector k = (12120) below TN∼ 17 K. Scattering
from both the Nd and Ir magnetic sublattices was required to
describe the data, and both were found to lie almost
completely within the ab plane. The dc susceptibility
revealed a bifurcation between the zero-field-cooled and
field-cooled curves below ∼13 K in Nd2ZnIrO6. A glassy
state was ruled out by ac susceptibility but detailed
magnetic isotherms revealed the opening of the loop below 13
K. These results suggest a delicate balance exists between
the Dzyaloshinskii-Moriya, crystal field schemes, and d-f
interaction in this series of compounds.},
cin = {JCNS-FRM-II / MLZ / JCNS-4},
ddc = {530},
cid = {I:(DE-Juel1)JCNS-FRM-II-20110218 / I:(DE-588b)4597118-3 /
I:(DE-Juel1)JCNS-4-20201012},
pnm = {6G4 - Jülich Centre for Neutron Research (JCNS) (FZJ)
(POF4-6G4) / 632 - Materials – Quantum, Complex and
Functional Materials (POF4-632)},
pid = {G:(DE-HGF)POF4-6G4 / G:(DE-HGF)POF4-632},
experiment = {EXP:(DE-MLZ)External-20140101},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000617788600005},
doi = {10.1103/PhysRevB.103.L060402},
url = {https://juser.fz-juelich.de/record/892554},
}