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@ARTICLE{Mauws:892557,
author = {Mauws, C. and Hiebert, N. and Rutherford, M. L. and Zhou,
H. D. and Huang, Q. and Stone, M. B. and Butch, N. P. and
Su, Yixi and Choi, E. S. and Yamani, Z. and Wiebe, C. R.},
title = {{M}agnetic ordering in the {I}sing antiferromagnetic
pyrochlore {N}d 2 {S}c{N}b{O} 7},
journal = {Journal of physics / Condensed matter},
volume = {33},
number = {24},
issn = {1361-648X},
address = {Bristol},
publisher = {IOP Publ.},
reportid = {FZJ-2021-02156},
pages = {245802 -},
year = {2021},
abstract = {The question of structural disorder and its effects on
magnetism is relevant to a number of spin liquid candidate
materials. Although commonly thought of as a route to spin
glass behaviour, here we describe a system in which the
structural disorder results in long-range antiferromagnetic
order due to local symmetry breaking. Nd2ScNbO7 is shown to
have a dispersionless gapped excitation observed in other
neodymium pyrochlores below TN = 0.37 K through polarized
and inelastic neutron scattering. However the dispersing
spin waves are not observed. This excited mode is shown to
occur in only $14(2)\%$ of the neodymium ions through
spectroscopy and is consistent with total scattering
measurements as well as the magnitude of the dynamic moment
0.26(2) μB. The remaining magnetic species order completely
into the all-in all-out Ising antiferromagnetic structure.
This can be seen as a result of local symmetry breaking due
disordered Sc+3 and Nb+5 ions about the A-site. From this
work, it has been established that B-site disorder restores
the dipole-like behaviour of the Nd+3 ions compared to the
Nd2B2O7 parent series.},
cin = {JCNS-FRM-II / MLZ / JCNS-2 / JCNS-4},
ddc = {530},
cid = {I:(DE-Juel1)JCNS-FRM-II-20110218 / I:(DE-588b)4597118-3 /
I:(DE-Juel1)JCNS-2-20110106 / I:(DE-Juel1)JCNS-4-20201012},
pnm = {6G4 - Jülich Centre for Neutron Research (JCNS) (FZJ)
(POF4-6G4) / 632 - Materials – Quantum, Complex and
Functional Materials (POF4-632)},
pid = {G:(DE-HGF)POF4-6G4 / G:(DE-HGF)POF4-632},
experiment = {EXP:(DE-MLZ)DNS-20140101},
typ = {PUB:(DE-HGF)16},
pubmed = {33827056},
UT = {WOS:000649934700001},
doi = {10.1088/1361-648X/abf594},
url = {https://juser.fz-juelich.de/record/892557},
}