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@ARTICLE{Wang:892827,
author = {Wang, Yuqi and Arabi, Soroush and Kern, Klaus and Ternes,
Markus},
title = {{S}ymmetry mediated tunable molecular magnetism on a 2{D}
material},
journal = {Communications Physics},
volume = {4},
number = {1},
issn = {2399-3650},
address = {London},
publisher = {Springer Nature},
reportid = {FZJ-2021-02370},
pages = {103},
year = {2021},
abstract = {Symmetries in nanoscale structures can be decisive for
their structural, electronic, and magnetic properties,
particularly in systems with reduced dimensions. Here we
show that the symmetries of a flat metal-organic molecule
adsorbed on a transition metal dichalcogenide, a
2-dimensional layered material, have a dramatic effect on
the total spin and the intramolecular spin-spin
interactions. Using a scanning probe microscope, we find two
different molecular spin states by modifying the symmetry of
the molecules via the twist angle to the substrate.
Additionally, we observe significant non-collinear
Dzyaloshinskii–Moriya interaction between two electron
spins on the molecule induced by the spin-orbit coupling of
the van der Waals coupled layered material with broken
inversion symmetry. Our work opens a path for modifying the
spin by exploiting symmetries and for studying the nature of
surface-induced non-collinear spin-spin interaction within a
single molecule which might allow the realization of more
complex topological spin structures.},
cin = {PGI-3},
ddc = {530},
cid = {I:(DE-Juel1)PGI-3-20110106},
pnm = {521 - Quantum Materials (POF4-521)},
pid = {G:(DE-HGF)POF4-521},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000657764200002},
doi = {10.1038/s42005-021-00601-8},
url = {https://juser.fz-juelich.de/record/892827},
}