000892838 001__ 892838
000892838 005__ 20240618202015.0
000892838 0247_ $$2doi$$a10.3390/membranes11060413
000892838 0247_ $$2Handle$$a2128/27901
000892838 0247_ $$2pmid$$a34070912
000892838 0247_ $$2WOS$$aWOS:000666442200001
000892838 0247_ $$2altmetric$$aaltmetric:108543358
000892838 037__ $$aFZJ-2021-02377
000892838 082__ $$a570
000892838 1001_ $$0P:(DE-Juel1)130893$$aPipich, Vitaliy$$b0$$ufzj
000892838 245__ $$aSilica Fouling in Reverse Osmosis Systems–Operando Small-Angle Neutron Scattering Studies
000892838 260__ $$aBasel$$bMDPI$$c2021
000892838 3367_ $$2DRIVER$$aarticle
000892838 3367_ $$2DataCite$$aOutput Types/Journal article
000892838 3367_ $$0PUB:(DE-HGF)16$$2PUB:(DE-HGF)$$aJournal Article$$bjournal$$mjournal$$s1718703327_15434
000892838 3367_ $$2BibTeX$$aARTICLE
000892838 3367_ $$2ORCID$$aJOURNAL_ARTICLE
000892838 3367_ $$00$$2EndNote$$aJournal Article
000892838 520__ $$aWe present operando small-angle neutron scattering (SANS) experiments on silica fouling at two reverse osmose (RO) membranes under almost realistic conditions of practiced RO desalination technique. To its realization, two cells were designed for pressure fields and tangential feed cross-flows up to 50 bar and 36 L/h, one cell equipped with the membrane and the other one as an empty cell to measure the feed solution in parallel far from the membrane. We studied several aqueous silica dispersions combining the parameters of colloidal radius, volume fraction, and ionic strength. A relevant result is the observation of Bragg diffraction as part of the SANS scattering pattern, representing a crystalline cake layer of simple cubic lattice structure. Other relevant parameters are silica colloidal size and volume fraction far from and above the membrane, as well as the lattice parameter of the silica cake layer, its volume fraction, thickness, and porosity in comparison with the corresponding permeate flux. The experiments show that the formation of cake layer depends to a large extent on colloidal size, ionic strength and cross-flow. Cake layer formation proved to be a reversible process, which could be dissolved at larger cross-flow. Only in one case we observed an irreversible cake layer formation showing the characteristics of an unstable phase transition. We likewise observed enhanced silica concentration and/or cake formation above the membrane, giving indication of a first order liquid–solid phase transformation.
000892838 536__ $$0G:(DE-HGF)POF4-524$$a524 - Molecular and Cellular Information Processing (POF4-524)$$cPOF4-524$$fPOF IV$$x0
000892838 536__ $$0G:(DE-HGF)POF4-6G4$$a6G4 - Jülich Centre for Neutron Research (JCNS) (FZJ) (POF4-6G4)$$cPOF4-6G4$$fPOF IV$$x1
000892838 536__ $$0G:(DE-HGF)POF4-632$$a632 - Materials – Quantum, Complex and Functional Materials (POF4-632)$$cPOF4-632$$fPOF IV$$x2
000892838 536__ $$0G:(DE-HGF)POF4-5241$$a5241 - Molecular Information Processing in Cellular Systems (POF4-524)$$cPOF4-524$$fPOF IV$$x3
000892838 588__ $$aDataset connected to CrossRef, Journals: juser.fz-juelich.de
000892838 65027 $$0V:(DE-MLZ)SciArea-150$$2V:(DE-HGF)$$aIndustrial Application$$x0
000892838 65017 $$0V:(DE-MLZ)GC-170-2016$$2V:(DE-HGF)$$aEarth, Environment and Cultural Heritage$$x0
000892838 693__ $$0EXP:(DE-MLZ)KWS3-20140101$$1EXP:(DE-MLZ)FRMII-20140101$$5EXP:(DE-MLZ)KWS3-20140101$$6EXP:(DE-MLZ)NL3auS-20140101$$aForschungs-Neutronenquelle Heinz Maier-Leibnitz $$eKWS-3: Very small angle scattering diffractometer with focusing mirror$$fNL3auS$$x0
000892838 7001_ $$0P:(DE-Juel1)130983$$aStarc, Thomas$$b1$$ufzj
000892838 7001_ $$0P:(DE-Juel1)130577$$aBuitenhuis, Johan$$b2$$ufzj
000892838 7001_ $$0P:(DE-HGF)0$$aKasher, Roni$$b3
000892838 7001_ $$0P:(DE-Juel1)178724$$aPetry, Winfried$$b4
000892838 7001_ $$0P:(DE-HGF)0$$aOren, Yoram$$b5
000892838 7001_ $$0P:(DE-Juel1)130962$$aSchwahn, Dietmar$$b6$$eCorresponding author
000892838 773__ $$0PERI:(DE-600)2614641-1$$a10.3390/membranes11060413$$gVol. 11, no. 6, p. 413 -$$n6$$p413 -$$tMembranes$$v11$$x2077-0375$$y2021
000892838 8564_ $$uhttps://juser.fz-juelich.de/record/892838/files/Invoice_MDPI_membranes-1224631_1379.62EUR.pdf
000892838 8564_ $$uhttps://juser.fz-juelich.de/record/892838/files/membranes-11-00413.pdf$$yOpenAccess
000892838 8767_ $$81224631$$92021-05-27$$d2021-06-01$$eAPC$$jZahlung erfolgt$$zBelegnr. 1200167623
000892838 909CO $$ooai:juser.fz-juelich.de:892838$$pdnbdelivery$$popenCost$$pVDB$$pVDB:MLZ$$pdriver$$pOpenAPC$$popenaire$$popen_access
000892838 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)130893$$aForschungszentrum Jülich$$b0$$kFZJ
000892838 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)130983$$aForschungszentrum Jülich$$b1$$kFZJ
000892838 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)130577$$aForschungszentrum Jülich$$b2$$kFZJ
000892838 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)178724$$aForschungszentrum Jülich$$b4$$kFZJ
000892838 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)130962$$aForschungszentrum Jülich$$b6$$kFZJ
000892838 9131_ $$0G:(DE-HGF)POF4-524$$1G:(DE-HGF)POF4-520$$2G:(DE-HGF)POF4-500$$3G:(DE-HGF)POF4$$4G:(DE-HGF)POF$$aDE-HGF$$bKey Technologies$$lNatural, Artificial and Cognitive Information Processing$$vMolecular and Cellular Information Processing$$x0
000892838 9131_ $$0G:(DE-HGF)POF4-6G4$$1G:(DE-HGF)POF4-6G0$$2G:(DE-HGF)POF4-600$$3G:(DE-HGF)POF4$$4G:(DE-HGF)POF$$aDE-HGF$$bForschungsbereich Materie$$lGroßgeräte: Materie$$vJülich Centre for Neutron Research (JCNS) (FZJ)$$x1
000892838 9131_ $$0G:(DE-HGF)POF4-632$$1G:(DE-HGF)POF4-630$$2G:(DE-HGF)POF4-600$$3G:(DE-HGF)POF4$$4G:(DE-HGF)POF$$aDE-HGF$$bForschungsbereich Materie$$lVon Materie zu Materialien und Leben$$vMaterials – Quantum, Complex and Functional Materials$$x2
000892838 9131_ $$0G:(DE-HGF)POF4-524$$1G:(DE-HGF)POF4-520$$2G:(DE-HGF)POF4-500$$3G:(DE-HGF)POF4$$4G:(DE-HGF)POF$$9G:(DE-HGF)POF4-5241$$aDE-HGF$$bKey Technologies$$lNatural, Artificial and Cognitive Information Processing$$vMolecular and Cellular Information Processing$$x3
000892838 9130_ $$0G:(DE-HGF)POF3-551$$1G:(DE-HGF)POF3-550$$2G:(DE-HGF)POF3-500$$3G:(DE-HGF)POF3$$4G:(DE-HGF)POF$$aDE-HGF$$bKey Technologies$$lBioSoft – Fundamentals for future Technologies in the fields of Soft Matter and Life Sciences$$vFunctional Macromolecules and Complexes$$x0
000892838 9141_ $$y2021
000892838 915__ $$0StatID:(DE-HGF)0200$$2StatID$$aDBCoverage$$bSCOPUS$$d2020-09-02
000892838 915__ $$0StatID:(DE-HGF)0300$$2StatID$$aDBCoverage$$bMedline$$d2020-09-02
000892838 915__ $$0StatID:(DE-HGF)1160$$2StatID$$aDBCoverage$$bCurrent Contents - Engineering, Computing and Technology$$d2020-09-02
000892838 915__ $$0LIC:(DE-HGF)CCBY4$$2HGFVOC$$aCreative Commons Attribution CC BY 4.0
000892838 915__ $$0StatID:(DE-HGF)0600$$2StatID$$aDBCoverage$$bEbsco Academic Search$$d2020-09-02
000892838 915__ $$0StatID:(DE-HGF)1150$$2StatID$$aDBCoverage$$bCurrent Contents - Physical, Chemical and Earth Sciences$$d2020-09-02
000892838 915__ $$0StatID:(DE-HGF)0501$$2StatID$$aDBCoverage$$bDOAJ Seal$$d2020-09-02
000892838 915__ $$0StatID:(DE-HGF)0500$$2StatID$$aDBCoverage$$bDOAJ$$d2020-09-02
000892838 915__ $$0StatID:(DE-HGF)0113$$2StatID$$aWoS$$bScience Citation Index Expanded$$d2020-09-02
000892838 915__ $$0StatID:(DE-HGF)0199$$2StatID$$aDBCoverage$$bClarivate Analytics Master Journal List$$d2020-09-02
000892838 915__ $$0StatID:(DE-HGF)0150$$2StatID$$aDBCoverage$$bWeb of Science Core Collection$$d2020-09-02
000892838 915__ $$0StatID:(DE-HGF)0510$$2StatID$$aOpenAccess
000892838 915__ $$0StatID:(DE-HGF)0030$$2StatID$$aPeer Review$$bASC$$d2020-09-02
000892838 915__ $$0StatID:(DE-HGF)0561$$2StatID$$aArticle Processing Charges$$d2020-09-02
000892838 915__ $$0StatID:(DE-HGF)0160$$2StatID$$aDBCoverage$$bEssential Science Indicators$$d2020-09-02
000892838 915__ $$0StatID:(DE-HGF)0320$$2StatID$$aDBCoverage$$bPubMed Central$$d2020-09-02
000892838 915__ $$0StatID:(DE-HGF)0700$$2StatID$$aFees$$d2020-09-02
000892838 920__ $$lyes
000892838 9201_ $$0I:(DE-Juel1)JCNS-1-20110106$$kJCNS-1$$lNeutronenstreuung$$x0
000892838 9201_ $$0I:(DE-Juel1)IBI-4-20200312$$kIBI-4$$lBiomakromolekulare Systeme und Prozesse$$x1
000892838 9201_ $$0I:(DE-Juel1)JCNS-FRM-II-20110218$$kJCNS-FRM-II$$lJCNS-FRM-II$$x2
000892838 9201_ $$0I:(DE-588b)4597118-3$$kMLZ$$lHeinz Maier-Leibnitz Zentrum$$x3
000892838 9201_ $$0I:(DE-Juel1)JCNS-4-20201012$$kJCNS-4$$lJCNS-4$$x4
000892838 980__ $$ajournal
000892838 980__ $$aVDB
000892838 980__ $$aI:(DE-Juel1)JCNS-1-20110106
000892838 980__ $$aI:(DE-Juel1)IBI-4-20200312
000892838 980__ $$aI:(DE-Juel1)JCNS-FRM-II-20110218
000892838 980__ $$aI:(DE-588b)4597118-3
000892838 980__ $$aI:(DE-Juel1)JCNS-4-20201012
000892838 980__ $$aAPC
000892838 980__ $$aUNRESTRICTED
000892838 9801_ $$aAPC
000892838 9801_ $$aFullTexts