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@ARTICLE{Ihrig:892896,
author = {Ihrig, Martin and Mishra, Tarini Prasad and Scheld, Walter
Sebastian and Häuschen, Grit and Rheinheimer, Wolfgang and
Bram, Martin and Finsterbusch, Martin and Guillon, Olivier},
title = {{L}i7{L}a3{Z}r2{O}12 solid electrolyte sintered by the
ultrafast high-temperature method},
journal = {Journal of the European Ceramic Society},
volume = {41},
number = {12},
issn = {0955-2219},
address = {Amsterdam [u.a.]},
publisher = {Elsevier Science},
reportid = {FZJ-2021-02423},
pages = {6075-6079},
year = {2021},
note = {Die letzte Version existiert nur in der Fomatierung des
Verlages, daher kein Post Print},
abstract = {All-solid-state Li batteries (ASSLBs) are regarded as the
systems of choice for future electrochemical energy storage.
Particularly, the garnet Li7La3Zr2O12 (LLZO) is one of the
most promising solid electrolytes due to its stability
against Li metal. However, its integration into ASSLBs is
challenging due to high temperature and long dwell time
required for sintering. Advanced sintering techniques, such
as Ultrafast High-temperature Sintering, have shown to
significantly increase the sintering rate. Direct contact to
graphite heaters allows sintering of LLZO within 10 s due to
extremely high heating rates (up to 104 K min−1) and
temperatures up to 1500 °C to a density around 80 $\%.$ The
LLZO sintered in vacuum and Ar atmosphere has good
mechanical stability and high phase purity, but kinetic
de-mixing at the grain boundaries was observed.
Nevertheless, the Li-ion conductivity of 1 mS cm−1 at 80
°C was comparable to conventional sintering, but lower than
for Field-Assisted Sintering Technique/Spark Plasma
Sintering.},
cin = {IEK-1 / JARA-ENERGY},
ddc = {660},
cid = {I:(DE-Juel1)IEK-1-20101013 / $I:(DE-82)080011_20140620$},
pnm = {1221 - Fundamentals and Materials (POF4-122)},
pid = {G:(DE-HGF)POF4-1221},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000661435800002},
doi = {10.1016/j.jeurceramsoc.2021.05.041},
url = {https://juser.fz-juelich.de/record/892896},
}