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@PHDTHESIS{Hoppe:893047,
author = {Hoppe, Eugen},
title = {{K}ompressionseigenschaften der {G}asdiffusionslage einer
{H}ochtemperatur-{P}olymerelektrolyt-{B}rennstoffzelle},
volume = {537},
school = {RWTH Aachen University},
type = {Dissertation},
address = {Jülich},
publisher = {Forschungszentrum Jülich GmbH Zentralbibliothek, Verlag},
reportid = {FZJ-2021-02525},
isbn = {978-3-95806-549-9},
series = {Schriften des Forschungszentrums Jülich Reihe Energie $\&$
Umwelt / Energy $\&$ Environment},
pages = {viii, 153},
year = {2021},
note = {Dissertation, RWTH Aachen University, 2021},
abstract = {The high-temperature polymer electrolyte fuel cell
(HT-PEFC) has a wide range of applicationsin stationary
applications such as combined heat and power generation or
as uninterruptiblepower supply, as well as on-board power
supply in mobile applications.The aim of the present work is
to investigate the compression behavior of the gas diffusion
layer(GDL) used in an HT-PEFC in combination with the
membrane electrode assembly (MEA). Tocharacterize the
compression behavior, the parameters porosity, permeability
and the intrusionbehavior of the GDL into the flow channel
are used. Using a computer tomograph, 3D modelsof the
compressed GDL are generated in the MEA assembly and the
relevant parameters aredetermined in post-processing. Based
on the obtained properties of the compressed GDL,
HTPEFCsingle cell tests are carried out with two commercial
MEAs to show the influence of thechange in properties of the
GDL on cell performance.For the ex-situ tests, three
different GDL types, namely H2315 C2 from Freudenberg FCCT
$SE\&$ Co. KG (non-woven), TGP-H-060 from Toray Industries
Inc. (paper) and AvCarb 1071HCB(woven) from AvCarb Material
Solutions were used. In a first compression cell, the GDLs
in theMEA assembly are compressed by a one-sided channel-rib
structure with channel widths of0;8 and 1;0 mm, and the
porosity, as well as the penetration behavior and
permeability are determined.The non-woven and paper GDLs
show an equivalent behavior both on the changingcompression
and on the variation of the channel width. Regardless of the
channel width, theporosity of the three GDLs decreases
linearly. Against the background of manufacturing
andassembly tolerances, the influence of the flowfield plate
misalignment on the intrusion behaviorin five channel pairs
was investigated in a second compression cell with constant
compression.As the misalignment increases, the point of
maximum intrusion depth also shifts and thecatalyst coated
membrane (CCM) moves towards the channels.The single cell
experiments with varying compression show that for a maximum
power density,compressions of up to $15\%$ can be selected
for the MEA with non-woven GDL and up $to20\%$ for the MEA
with woven GDL. A misalignment of the flowfield plates by
almost $50\%(1$ mm) has no significant influence on the
performance of an HT-PEFC single cell for bothMEAs
investigated.},
cin = {IEK-14},
cid = {I:(DE-Juel1)IEK-14-20191129},
pnm = {1231 - Electrochemistry for Hydrogen (POF4-123)},
pid = {G:(DE-HGF)POF4-1231},
typ = {PUB:(DE-HGF)3 / PUB:(DE-HGF)11},
urn = {urn:nbn:de:0001-2021072207},
url = {https://juser.fz-juelich.de/record/893047},
}