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000894123 1001_ $$0P:(DE-Juel1)178813$$aWellmann, Julia$$b0
000894123 245__ $$aEffective Solid Electrolyte Interphase Formation on Lithium Metal Anodes by Mechanochemical Modification
000894123 260__ $$aWashington, DC$$bSoc.$$c2021
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000894123 520__ $$aLithium metal batteries are gaining increasing attention due to their potential for significantly higher theoretical energy density than conventional lithium ion batteries. Here, we present a novel mechanochemical modification method for lithium metal anodes, involving roll-pressing the lithium metal foil in contact with ionic liquid-based solutions, enabling the formation of an artificial solid electrolyte interphase with favorable properties such as an improved lithium ion transport and, most importantly, the suppression of dendrite growth, allowing homogeneous electrodeposition/-dissolution using conventional and highly conductive room temperature alkyl carbonate-based electrolytes. As a result, stable cycling in symmetrical Li∥Li cells is achieved even at a high current density of 10 mA cm–2. Furthermore, the rate capability and the capacity retention in NMC∥Li cells are significantly improved.
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000894123 536__ $$0G:(EU-Grant)814389$$aSPIDER - Safe and Prelithiated hIgh energy DEnsity batteries based on sulphur Rocksalt and silicon chemistries (814389)$$c814389$$fH2020-NMBP-ST-IND-2018$$x1
000894123 536__ $$0G:(EU-Grant)829145$$aVIDICAT - Versatile Ionomers for DIvalent CAlcium baTteries (829145)$$c829145$$fH2020-FETOPEN-2018-2019-2020-01$$x2
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000894123 7001_ $$0P:(DE-Juel1)176761$$aBrinkmann, Jan-Paul$$b1$$ufzj
000894123 7001_ $$0P:(DE-HGF)0$$aWankmiller, Björn$$b2
000894123 7001_ $$0P:(DE-Juel1)181017$$aNeuhaus, Kerstin$$b3$$ufzj
000894123 7001_ $$0P:(DE-Juel1)178947$$aRodehorst, Uta$$b4$$ufzj
000894123 7001_ $$00000-0001-7114-8051$$aHansen, Michael R.$$b5
000894123 7001_ $$0P:(DE-Juel1)166130$$aWinter, Martin$$b6$$ufzj
000894123 7001_ $$0P:(DE-Juel1)166311$$aPaillard, Elie$$b7$$eCorresponding author
000894123 773__ $$0PERI:(DE-600)2467494-1$$a10.1021/acsami.1c07490$$gp. acsami.1c07490$$n29$$p34227–34237$$tACS applied materials & interfaces$$v13$$x1944-8244$$y2021
000894123 8564_ $$uhttps://pubs.acs.org/doi/full/10.1021/acsami.1c07490
000894123 8564_ $$uhttps://juser.fz-juelich.de/record/894123/files/am-2021-07490j_Main_Manuscript_2ndRevision.pdf$$yPublished on 2021-07-15. Available in OpenAccess from 2022-07-15.
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