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@ARTICLE{Wellmann:894123,
author = {Wellmann, Julia and Brinkmann, Jan-Paul and Wankmiller,
Björn and Neuhaus, Kerstin and Rodehorst, Uta and Hansen,
Michael R. and Winter, Martin and Paillard, Elie},
title = {{E}ffective {S}olid {E}lectrolyte {I}nterphase {F}ormation
on {L}ithium {M}etal {A}nodes by {M}echanochemical
{M}odification},
journal = {ACS applied materials $\&$ interfaces},
volume = {13},
number = {29},
issn = {1944-8244},
address = {Washington, DC},
publisher = {Soc.},
reportid = {FZJ-2021-03050},
pages = {34227–34237},
year = {2021},
abstract = {Lithium metal batteries are gaining increasing attention
due to their potential for significantly higher theoretical
energy density than conventional lithium ion batteries.
Here, we present a novel mechanochemical modification method
for lithium metal anodes, involving roll-pressing the
lithium metal foil in contact with ionic liquid-based
solutions, enabling the formation of an artificial solid
electrolyte interphase with favorable properties such as an
improved lithium ion transport and, most importantly, the
suppression of dendrite growth, allowing homogeneous
electrodeposition/-dissolution using conventional and highly
conductive room temperature alkyl carbonate-based
electrolytes. As a result, stable cycling in symmetrical
Li∥Li cells is achieved even at a high current density of
10 mA cm–2. Furthermore, the rate capability and the
capacity retention in NMC∥Li cells are significantly
improved.},
cin = {IEK-12},
ddc = {600},
cid = {I:(DE-Juel1)IEK-12-20141217},
pnm = {1221 - Fundamentals and Materials (POF4-122) / SPIDER -
Safe and Prelithiated hIgh energy DEnsity batteries based on
sulphur Rocksalt and silicon chemistries (814389) / VIDICAT
- Versatile Ionomers for DIvalent CAlcium baTteries
(829145)},
pid = {G:(DE-HGF)POF4-1221 / G:(EU-Grant)814389 /
G:(EU-Grant)829145},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:34264641},
UT = {WOS:000679917500047},
doi = {10.1021/acsami.1c07490},
url = {https://juser.fz-juelich.de/record/894123},
}