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@ARTICLE{Bressi:894239,
author = {Bressi, M. and Cavalli, F. and Putaud, J. P. and Fröhlich,
R. and Petit, J.-E. and Aas, W. and Äijälä, M. and
Alastuey, A. and Allan, J. D. and Aurela, M. and Berico, M.
and Bougiatioti, A. and Bukowiecki, N. and Canonaco, F. and
Crenn, V. and Dusanter, S. and Ehn, M. and Elsasser, M. and
Flentje, H. and Graf, P. and Green, D. C. and Heikkinen, L.
and Hermann, H. and Holzinger, R. and Hueglin, C. and
Keernik, H. and Kiendler-Scharr, A. and Kubelová, L. and
Lunder, C. and Maasikmets, M. and Makeš, O. and Malaguti,
A. and Mihalopoulos, N. and Nicolas, J. B. and O'Dowd, C.
and Ovadnevaite, J. and Petralia, E. and Poulain, L. and
Priestman, M. and Riffault, V. and Ripoll, A. and Schlag, P.
and Schwarz, J. and Sciare, J. and Slowik, J. and Sosedova,
Y. and Stavroulas, I. and Teinemaa, E. and Via, M. and
Vodička, P. and Williams, P. I. and Wiedensohler, A. and
Young, D. E. and Zhang, S. and Favez, O. and Minguillón, M.
C. and Prevot, A. S. H.},
title = {{A} {E}uropean aerosol phenomenology - 7: {H}igh-time
resolution chemical characteristics of submicron particulate
matter across {E}urope},
journal = {Atmospheric environment: X},
volume = {10},
issn = {2590-1621},
address = {Amsterdam},
publisher = {Elsevier},
reportid = {FZJ-2021-03119},
pages = {100108 -},
year = {2021},
abstract = {Similarities and differences in the submicron atmospheric
aerosol chemical composition are analyzed from a unique set
of measurements performed at 21 sites across Europe for at
least one year. These sites are located between 35 and 62°N
and 10° W – 26°E, and represent various types of
settings (remote, coastal, rural, industrial, urban).
Measurements were all carried out on-line with a 30-min time
resolution using mass spectroscopy based instruments known
as Aerosol Chemical Speciation Monitors (ACSM) and Aerosol
Mass Spectrometers (AMS) and following common measurement
guidelines. Data regarding organics, sulfate, nitrate and
ammonium concentrations, as well as the sum of them called
non-refractory submicron aerosol mass concentration
([NR-PM1]) are discussed. NR-PM1 concentrations generally
increase from remote to urban sites. They are mostly larger
in the mid-latitude band than in southern and northern
Europe. On average, organics account for the major part
$(36–64\%)$ of NR-PM1 followed by sulfate $(12–44\%)$
and nitrate $(6–35\%).$ The annual mean chemical
composition of NR-PM1 at rural (or regional background)
sites and urban background sites are very similar.
Considering rural and regional background sites only,
nitrate contribution is higher and sulfate contribution is
lower in mid-latitude Europe compared to northern and
southern Europe. Large seasonal variations in concentrations
(μg/m³) of one or more components of NR-PM1 can be
observed at all sites, as well as in the chemical
composition of NR-PM1 $(\%)$ at most sites. Significant diel
cycles in the contribution to [NR-PM1] of organics, sulfate,
and nitrate can be observed at a majority of sites both in
winter and summer. Early morning minima in organics in
concomitance with maxima in nitrate are common features at
regional and urban background sites. Daily variations are
much smaller at a number of coastal and rural sites. Looking
at NR-PM1 chemical composition as a function of NR-PM1 mass
concentration reveals that although organics account for the
major fraction of NR-PM1 at all concentration levels at most
sites, nitrate contribution generally increases with NR-PM1
mass concentration and predominates when NR-PM1 mass
concentrations exceed 40 μg/m³ at half of the sites.},
cin = {IEK-8},
ddc = {550},
cid = {I:(DE-Juel1)IEK-8-20101013},
pnm = {2111 - Air Quality (POF4-211)},
pid = {G:(DE-HGF)POF4-2111},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000660094500004},
doi = {10.1016/j.aeaoa.2021.100108},
url = {https://juser.fz-juelich.de/record/894239},
}