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000894440 1001_ $$00000-0003-4506-6727$$aDiekmann, Jonas$$b0
000894440 245__ $$aPathways toward 30% Efficient Single‐Junction Perovskite Solar Cells and the Role of Mobile Ions
000894440 260__ $$aWeinheim$$bWiley-VCH$$c2021
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000894440 520__ $$aPerovskite semiconductors have demonstrated outstanding external luminescence quantum yields, enabling high power conversion efficiencies (PCEs). However, the precise conditions to advance to an efficiency regime above monocrystalline silicon cells are not well understood. Herein, a simulation model that describes efficient p–i–n-type perovskite solar cells well and a range of different experiments is established. Then, important device and material parameters are studied and it is found that an efficiency regime of 30% can be unlocked by optimizing the built-in voltage across the perovskite layer using either highly doped (1019 cm−3) transport layers (TLs), doped interlayers or ultrathin self-assembled monolayers. Importantly, only parameters that have been reported in recent literature are considered, that is, a bulk lifetime of 10 μs, interfacial recombination velocities of 10 cm s−1, a perovskite bandgap ( 
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000894440 7001_ $$0P:(DE-HGF)0$$aCaprioglio, Pietro$$b1
000894440 7001_ $$0P:(DE-HGF)0$$aFutscher, Moritz H.$$b2
000894440 7001_ $$0P:(DE-HGF)0$$aLe Corre, Vincent M.$$b3
000894440 7001_ $$0P:(DE-HGF)0$$aReichert, Sebastian$$b4
000894440 7001_ $$0P:(DE-HGF)0$$aJaiser, Frank$$b5
000894440 7001_ $$0P:(DE-HGF)0$$aArvind, Malavika$$b6
000894440 7001_ $$0P:(DE-HGF)0$$aToro, Lorena Perdigón$$b7
000894440 7001_ $$0P:(DE-HGF)0$$aGutierrez-Partida, Emilio$$b8
000894440 7001_ $$0P:(DE-HGF)0$$aPeña-Camargo, Francisco$$b9
000894440 7001_ $$0P:(DE-HGF)0$$aDeibel, Carsten$$b10
000894440 7001_ $$0P:(DE-HGF)0$$aEhrler, Bruno$$b11
000894440 7001_ $$0P:(DE-HGF)0$$aUnold, Thomas$$b12
000894440 7001_ $$0P:(DE-Juel1)159457$$aKirchartz, Thomas$$b13$$ufzj
000894440 7001_ $$0P:(DE-HGF)0$$aNeher, Dieter$$b14
000894440 7001_ $$00000-0002-4023-2178$$aStolterfoht, Martin$$b15$$eCorresponding author
000894440 773__ $$0PERI:(DE-600)2882014-9$$a10.1002/solr.202100219$$gVol. 5, no. 8, p. 2100219 -$$n8$$p2100219$$tSolar RRL$$v5$$x2367-198X$$y2021
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