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001     894719
005     20220131120401.0
024 7 _ |a 10.3762/bjnano.11.132
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024 7 _ |a 2128/28591
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100 1 _ |a Hurdax, Philipp
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245 _ _ |a Controlling the electronic and physical coupling on dielectric thin films
260 _ _ |a Frankfurt, M.
|c 2020
|b Beilstein-Institut zur Förderung der Chemischen Wissenschaften
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520 _ _ |a Ultrathin dielectric/insulating films on metals are often used as decoupling layers to allow for the study of the electronic properties of adsorbed molecules without electronic interference from the underlying metal substrate. However, the presence of such decoupling layers may effectively change the electron donating properties of the substrate, for example, by lowering its work function and thus enhancing the charging of the molecular adsorbate layer through electron tunneling. Here, an experimental study of the charging of para-sexiphenyl (6P) on ultrathin MgO(100) films supported on Ag(100) is reported. By deliberately changing the work function of the MgO(100)/Ag(100) system, it is shown that the charge transfer (electronic coupling) into the 6P molecules can be controlled, and 6P monolayers with uncharged molecules (Schottky–Mott regime) and charged and uncharged molecules (Fermi level pinning regime) can be obtained. Furthermore, it was found that charge transfer and temperature strongly influence the orientation, conformation, and wetting behavior (physical coupling) of the 6P layers on the MgO(100) thin films.
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700 1 _ |a Hollerer, Michael
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700 1 _ |a Egger, Larissa
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700 1 _ |a Koller, Georg
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700 1 _ |a Yang, Xiaosheng
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700 1 _ |a Haags, Anja
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700 1 _ |a Soubatch, Serguei
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700 1 _ |a Tautz, Frank Stefan
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700 1 _ |a Richter, Mathias
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700 1 _ |a Gottwald, Alexander
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700 1 _ |a Puschnig, Peter
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700 1 _ |a Sterrer, Martin
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700 1 _ |a Ramsey, Michael G
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773 _ _ |a 10.3762/bjnano.11.132
|g Vol. 11, p. 1492 - 1503
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|t Beilstein journal of nanotechnology
|v 11
|y 2020
|x 2190-4286
856 4 _ |u https://juser.fz-juelich.de/record/894719/files/2190-4286-11-132.pdf
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