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@ARTICLE{Blowey:894721,
author = {Blowey, P. J. and Haags, A. and Rochford, L. A. and Felter,
J. and Warr, D. A. and Duncan, D. A. and Lee, T.-L. and
Costantini, G. and Kumpf, C. and Woodruff, D. P.},
title = {{C}haracterization of growth and structure of {TCNQ} phases
on {A}g(111)},
journal = {Physical review materials},
volume = {3},
number = {11},
issn = {2475-9953},
address = {College Park, MD},
publisher = {APS},
reportid = {FZJ-2021-03373},
pages = {116001},
year = {2019},
abstract = {A combination of scanning tunneling microscopy, low-energy
electron diffraction,and low-energy electron microscopy
(LEEM) has been used to identify the structural phases
formed by 7,7,8,8-tetracyanoquinodimethane (TCNQ) on
Ag(111). These comprise a two-dimensional gas phase, a
low-density commensurate (LDC) phase, and a higher-density
incommensurate (HDI) phase. LEEM also shows the presence of
an additional “precursor-HDI” phase with a surface unit
mesh area only $≈3\%$ less than the HDI phase. Normal
incidence x-ray standing-wave measurements of the HDI phase
yield almost identical structural parameters to the LDC
phase for which a full structure determination has been
previously reported. The results show TCNQ does not adopt
the inverted bowl distortion favored in earlier density
functional theory calculations of TCNQ on coinage metal
surfaces, but the N atoms are twisted out of the molecular
plane, an effect found for the LDC phase to be due to
incorporation of Ag adatoms. The possible role of Ag adatoms
in the HDI phase, and in the transition from the
precursor-HDI phase, is discussed.},
cin = {PGI-3},
ddc = {530},
cid = {I:(DE-Juel1)PGI-3-20110106},
pnm = {5213 - Quantum Nanoscience (POF4-521)},
pid = {G:(DE-HGF)POF4-5213},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000494462100002},
doi = {10.1103/PhysRevMaterials.3.116001},
url = {https://juser.fz-juelich.de/record/894721},
}