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@ARTICLE{Boukhvalov:894768,
      author       = {Boukhvalov, Danil W. and Cheng, Jia and D’Olimpio,
                      Gianluca and Bocquet, François C. and Kuo, Chia-Nung and
                      Sarkar, Anan Bari and Ghosh, Barun and Vobornik, Ivana and
                      Fujii, Jun and Hsu, Kuan and Wang, Li-Min and Azulay, Ori
                      and Daptary, Gopi Nath and Naveh, Doron and Lue, Chin Shan
                      and Vorokhta, Mykhailo and Agarwal, Amit and Zhang, Lixue
                      and Politano, Antonio},
      title        = {{U}nveiling the {M}echanisms {R}uling the {E}fficient
                      {H}ydrogen {E}volution {R}eaction with {M}itrofanovite {P}t
                      3 {T}e 4},
      journal      = {The journal of physical chemistry letters},
      volume       = {12},
      number       = {35},
      issn         = {1948-7185},
      address      = {Washington, DC},
      publisher    = {ACS},
      reportid     = {FZJ-2021-03382},
      pages        = {8627 - 8636},
      year         = {2021},
      abstract     = {By means of electrocatalytic tests, surface-science
                      techniques and density functional theory, we unveil the
                      physicochemical mechanisms ruling the electrocatalytic
                      activity of recently discovered mitrofanovite (Pt3Te4)
                      mineral. Mitrofanovite represents a very promising
                      electrocatalyst candidate for energy-related applications,
                      with a reduction of costs by $47\%$ compared to pure Pt and
                      superior robustness to CO poisoning. We show that Pt3Te4 is
                      a weak topological metal with the Z2 invariant, exhibiting
                      electrical conductivity (∼4 × 106 S/m) comparable with
                      pure Pt. In hydrogen evolution reaction (HER), the electrode
                      based on bulk Pt3Te4 shows a very small overpotential of 46
                      mV at 10 mA cm–2 and a Tafel slope of 36–49 mV dec–1
                      associated with the Volmer–Heyrovsky mechanism. The
                      outstanding ambient stability of Pt3Te4 also provides
                      durability of the electrode and long-term stability of its
                      efficient catalytic performances.},
      cin          = {PGI-3},
      ddc          = {530},
      cid          = {I:(DE-Juel1)PGI-3-20110106},
      pnm          = {5213 - Quantum Nanoscience (POF4-521) / DFG project
                      396769409 - Grundlagen der Photoemissionstomographie},
      pid          = {G:(DE-HGF)POF4-5213 / G:(GEPRIS)396769409},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {pmid:34472339},
      UT           = {WOS:000696175700025},
      doi          = {10.1021/acs.jpclett.1c01261},
      url          = {https://juser.fz-juelich.de/record/894768},
}