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@ARTICLE{Kalikka:894892,
author = {Kalikka, J. and Konstantinou, K. and Akola, J. and Jones,
Robert O.},
title = {{M}elt-quenched and as-deposited structures of amorphous
selenium: a density functional/ molecular dynamics
comparison},
journal = {Journal of physics / Condensed matter},
volume = {33},
number = {44},
issn = {1361-648X},
address = {Bristol},
publisher = {IOP Publ.},
reportid = {FZJ-2021-03458},
pages = {445401},
year = {2021},
abstract = {Molecular dynamics simulations using a density functional
description of energies and forces have been carried out for
a model of an as-deposited (AD) surface of amorphous
selenium. The deposition model assumed the annealing (at 400
K) of layers of randomly located single atoms, followed by
compression to the density used in earlier melt-quenched
(MQ) simulations of amorphous Se, and by further annealing.
The AD and MQ structures are predominantly twofold
coordinated and similar, for example in the pair
distribution functions, with notable differences: the AD
structures have more defects (atoms with one and three
neighbours), and the ring distributions differ. These
differences are also reflected in the electronic structures
of the AD and MQ samples, where the increased presence of
defects in the former influences the Bader charges and the
edge states of the band gap. The dominance of rings found in
a previous simulation of AD structures is not found.},
cin = {IAS-1 / PGI-1},
ddc = {530},
cid = {I:(DE-Juel1)IAS-1-20090406 / I:(DE-Juel1)PGI-1-20110106},
pnm = {5211 - Topological Matter (POF4-521)},
pid = {G:(DE-HGF)POF4-5211},
typ = {PUB:(DE-HGF)16},
pubmed = {34348254},
UT = {WOS:000687395100001},
doi = {10.1088/1361-648X/ac1aa3},
url = {https://juser.fz-juelich.de/record/894892},
}