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000897121 037__ $$aFZJ-2021-03619
000897121 1001_ $$0P:(DE-Juel1)176326$$aThoma, Henrik$$b0$$eCorresponding author$$ufzj
000897121 1112_ $$aXXV General Assembly and Congress of the International Union of Crystallography$$cPrague$$d2021-08-14 - 2021-08-22$$gIUCr 2021$$wCzech Republic
000897121 245__ $$aAbsolute sign of the Dzyaloshinskii-Moriya interaction in weak ferromagnets disclosed by polarized neutron diffraction
000897121 260__ $$c2021
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000897121 520__ $$aMagnetic interactions are the fundamental components for the fascinating variety of complex magnetic structures and properties found in many functional materials. Identifying, understanding, and finally predicting these interactions is an essential step towards their utilization in novel devices. One of these basic interactions is the Dzyaloshinskii-Moriya interaction (DMI) – an antisymmetric exchange coupling favouring a perpendicular arrangement of magnetic moments, and thus a canting in otherwise collinear structures [1,2]. The DMI, originally introduced in the late 1950s to explain ‘weak ferromagnets’ (not perfectly collinear antiferromagnets), regained the interest in current condensed matter research as it was found to be the driving force to stabilize various novel topological noncollinear magnetic structures, such as spin spirals [3], magnetic skyrmions [4], magnetic soliton lattices [5] and others. In particular for spintronic applications, the DMI shows promising characteristics towards the development of next-generation devices [6]. Although the magnitude of the DMI-induced canting is usually small, the direction can have a fundamental impact on the spin chirality and the resulting magnetic and multiferroic properties [7]. Here, we present polarized neutron diffraction (PND) as an efficient technique for the determination of the absolute direction of the DMI in weak ferromagnetic materials, as recently established by us [8]. We provide the basic formalism for a symmetry analysis of the DMI in crystal structures and show how to relate the measured PND data with the absolute DMI direction. We exemplify this approach in weak ferromagnetic MnCO3 and identify the magnetic moment configurations for a positive or negative sign of the DMI with an applied magnetic field. Using PND [9], we can distinguish even from the measurement of a single suitable Bragg reflection between the two configurations and unambiguously reveal a negative DMI sign in MnCO3. This is in agreement with previous results obtained by resonant magnetic X-ray scattering and thus, validates the method [10]. We demonstrate the generality of our method by providing further examples of topical magnetic materials with different symmetries and support our findings with ab-initio calculations, which reproduce the experimental results. [1] V. E. Dzyaloshinskii, Sov. Phys. - JETP 5(6), 1259 (1957)[2] T. Moriya, Phys. Rev. 120(1), 91 (1960),[3] M. Bode et al., Nature 447, 190 (2007),[4] S. Heinze et al., Nat. Phys. 7, 713 (2011),[5] Y. Togawa et al., Phys. Rev. Lett. 108, 107202 (2012),[6] S. S. P. Parkin et al., Science 320, 190 (2008),[7] J. Cho et al., J. Phys. D: Appl. Phys. 50, 425004 (2017),[8] H. Thoma et al., Phys. Rev. X 11, 011060 (2021),[9] H. Thoma et al., J. Appl. Crystallogr. 51, 17 (2018),[10] V.  E.  Dmitrienko et al., Nat. Phys. 10, 202 (2014)
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000897121 65017 $$0V:(DE-MLZ)GC-1604-2016$$2V:(DE-HGF)$$aMagnetic Materials$$x0
000897121 65017 $$0V:(DE-MLZ)GC-2002-2016$$2V:(DE-HGF)$$aInstrument and Method Development$$x1
000897121 693__ $$0EXP:(DE-MLZ)POLI-HEIDI-20140101$$1EXP:(DE-MLZ)FRMII-20140101$$5EXP:(DE-MLZ)POLI-HEIDI-20140101$$6EXP:(DE-MLZ)SR9a-20140101$$aForschungs-Neutronenquelle Heinz Maier-Leibnitz $$ePOLI: Polarized hot neutron diffractometer$$fSR9a$$x0
000897121 7001_ $$0P:(DE-Juel1)164298$$aHutanu, Vladimir$$b1$$ufzj
000897121 7001_ $$0P:(DE-Juel1)130504$$aAngst, Manuel$$b2$$ufzj
000897121 7001_ $$0P:(DE-HGF)0$$aRoth, Georg$$b3
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