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000897473 1001_ $$0P:(DE-HGF)0$$aŽivković, Ivica$$b0$$eCorresponding author
000897473 245__ $$aMagnetic Field Induced Quantum Spin Liquid in the Two Coupled Trillium Lattices of K$_2$Ni$_2$(SO$_4$)$_3$
000897473 260__ $$aCollege Park, Md.$$bAPS$$c2021
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000897473 520__ $$aQuantum spin liquids are exotic states of matter that form when strongly frustrated magnetic interactions induce a highly entangled quantum paramagnet far below the energy scale of the magnetic interactions. Three-dimensional cases are especially challenging due to the significant reduction of the influence of quantum fluctuations. Here, we report the magnetic characterization of K2Ni2(SO4)3 forming a three-dimensional network of Ni2+ spins. Using density functional theory calculations, we show that this network consists of two interconnected spin-1 trillium lattices. In the absence of a magnetic field, magnetization, specific heat, neutron scattering, and muon spin relaxation experiments demonstrate a highly correlated and dynamic state, coexisting with a peculiar, very small static component exhibiting a strongly renormalized moment. A magnetic field B≳4  T diminishes the ordered component and drives the system into a pure quantum spin liquid state. This shows that a system of interconnected S=1 trillium lattices exhibits a significantly elevated level of geometrical frustration.
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000897473 65017 $$0V:(DE-MLZ)GC-1604-2016$$2V:(DE-HGF)$$aMagnetic Materials$$x0
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000897473 7001_ $$0P:(DE-HGF)0$$aFavre, Virgile$$b1
000897473 7001_ $$0P:(DE-HGF)0$$aSalazar Mejia, Catalina$$b2
000897473 7001_ $$0P:(DE-HGF)0$$aJeschke, Harald O.$$b3
000897473 7001_ $$0P:(DE-HGF)0$$aMagrez, Arnaud$$b4
000897473 7001_ $$0P:(DE-HGF)0$$aDabholkar, Bhupen$$b5
000897473 7001_ $$0P:(DE-HGF)0$$aNoculak, Vincent$$b6
000897473 7001_ $$0P:(DE-HGF)0$$aFreitas, Rafael S.$$b7
000897473 7001_ $$0P:(DE-HGF)0$$aJeong, Minki$$b8
000897473 7001_ $$0P:(DE-HGF)0$$aHegde, Nagabhushan G.$$b9
000897473 7001_ $$0P:(DE-HGF)0$$aTesta, Luc$$b10
000897473 7001_ $$0P:(DE-HGF)0$$aBabkevich, Peter$$b11
000897473 7001_ $$0P:(DE-Juel1)130991$$aSu, Yixi$$b12
000897473 7001_ $$0P:(DE-HGF)0$$aManuel, Pascal$$b13
000897473 7001_ $$0P:(DE-HGF)0$$aLuetkens, Hubertus$$b14
000897473 7001_ $$0P:(DE-HGF)0$$aBaines, Christopher$$b15
000897473 7001_ $$0P:(DE-HGF)0$$aBaker, Peter J.$$b16
000897473 7001_ $$0P:(DE-HGF)0$$aWosnitza, Jochen$$b17
000897473 7001_ $$0P:(DE-HGF)0$$aZaharko, Oksana$$b18
000897473 7001_ $$0P:(DE-HGF)0$$aIqbal, Yasir$$b19
000897473 7001_ $$0P:(DE-HGF)0$$aReuther, Johannes$$b20
000897473 7001_ $$0P:(DE-HGF)0$$aRønnow, Henrik M.$$b21
000897473 773__ $$0PERI:(DE-600)1472655-5$$a10.1103/PhysRevLett.127.157204$$gVol. 127, no. 15, p. 157204$$n15$$p157204$$tPhysical review letters$$v127$$x1079-7114$$y2021
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