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@ARTICLE{ivkovi:897473,
author = {Živković, Ivica and Favre, Virgile and Salazar Mejia,
Catalina and Jeschke, Harald O. and Magrez, Arnaud and
Dabholkar, Bhupen and Noculak, Vincent and Freitas, Rafael
S. and Jeong, Minki and Hegde, Nagabhushan G. and Testa, Luc
and Babkevich, Peter and Su, Yixi and Manuel, Pascal and
Luetkens, Hubertus and Baines, Christopher and Baker, Peter
J. and Wosnitza, Jochen and Zaharko, Oksana and Iqbal, Yasir
and Reuther, Johannes and Rønnow, Henrik M.},
title = {{M}agnetic {F}ield {I}nduced {Q}uantum {S}pin {L}iquid in
the {T}wo {C}oupled {T}rillium {L}attices of
{K}$_2${N}i$_2$({SO}$_4$)$_3$},
journal = {Physical review letters},
volume = {127},
number = {15},
issn = {1079-7114},
address = {College Park, Md.},
publisher = {APS},
reportid = {FZJ-2021-03806},
pages = {157204},
year = {2021},
abstract = {Quantum spin liquids are exotic states of matter that form
when strongly frustrated magnetic interactions induce a
highly entangled quantum paramagnet far below the energy
scale of the magnetic interactions. Three-dimensional cases
are especially challenging due to the significant reduction
of the influence of quantum fluctuations. Here, we report
the magnetic characterization of K2Ni2(SO4)3 forming a
three-dimensional network of Ni2+ spins. Using density
functional theory calculations, we show that this network
consists of two interconnected spin-1 trillium lattices. In
the absence of a magnetic field, magnetization, specific
heat, neutron scattering, and muon spin relaxation
experiments demonstrate a highly correlated and dynamic
state, coexisting with a peculiar, very small static
component exhibiting a strongly renormalized moment. A
magnetic field B≳4 T diminishes the ordered component
and drives the system into a pure quantum spin liquid state.
This shows that a system of interconnected S=1 trillium
lattices exhibits a significantly elevated level of
geometrical frustration.},
cin = {JCNS-FRM-II / JCNS-2 / JCNS-4 / MLZ},
ddc = {530},
cid = {I:(DE-Juel1)JCNS-FRM-II-20110218 /
I:(DE-Juel1)JCNS-2-20110106 / I:(DE-Juel1)JCNS-4-20201012 /
I:(DE-588b)4597118-3},
pnm = {6G4 - Jülich Centre for Neutron Research (JCNS) (FZJ)
(POF4-6G4) / 632 - Materials – Quantum, Complex and
Functional Materials (POF4-632)},
pid = {G:(DE-HGF)POF4-6G4 / G:(DE-HGF)POF4-632},
experiment = {EXP:(DE-MLZ)DNS-20140101},
typ = {PUB:(DE-HGF)16},
pubmed = {34677991},
UT = {WOS:000705651600013},
doi = {10.1103/PhysRevLett.127.157204},
url = {https://juser.fz-juelich.de/record/897473},
}