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| 001 | 897473 | ||
| 005 | 20220221143524.0 | ||
| 024 | 7 | _ | |a 10.1103/PhysRevLett.127.157204 |2 doi |
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| 100 | 1 | _ | |a Živković, Ivica |0 P:(DE-HGF)0 |b 0 |e Corresponding author |
| 245 | _ | _ | |a Magnetic Field Induced Quantum Spin Liquid in the Two Coupled Trillium Lattices of K$_2$Ni$_2$(SO$_4$)$_3$ |
| 260 | _ | _ | |a College Park, Md. |c 2021 |b APS |
| 336 | 7 | _ | |a article |2 DRIVER |
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| 520 | _ | _ | |a Quantum spin liquids are exotic states of matter that form when strongly frustrated magnetic interactions induce a highly entangled quantum paramagnet far below the energy scale of the magnetic interactions. Three-dimensional cases are especially challenging due to the significant reduction of the influence of quantum fluctuations. Here, we report the magnetic characterization of K2Ni2(SO4)3 forming a three-dimensional network of Ni2+ spins. Using density functional theory calculations, we show that this network consists of two interconnected spin-1 trillium lattices. In the absence of a magnetic field, magnetization, specific heat, neutron scattering, and muon spin relaxation experiments demonstrate a highly correlated and dynamic state, coexisting with a peculiar, very small static component exhibiting a strongly renormalized moment. A magnetic field B≳4 T diminishes the ordered component and drives the system into a pure quantum spin liquid state. This shows that a system of interconnected S=1 trillium lattices exhibits a significantly elevated level of geometrical frustration. |
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| 773 | _ | _ | |a 10.1103/PhysRevLett.127.157204 |g Vol. 127, no. 15, p. 157204 |0 PERI:(DE-600)1472655-5 |n 15 |p 157204 |t Physical review letters |v 127 |y 2021 |x 1079-7114 |
| 856 | 4 | _ | |u https://juser.fz-juelich.de/record/897473/files/PhysRevLett.127.157204.pdf |y OpenAccess |
| 856 | 4 | _ | |u https://juser.fz-juelich.de/record/897473/files/su_2109.04102.pdf |y OpenAccess |
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