000901867 001__ 901867
000901867 005__ 20230123110538.0
000901867 0247_ $$2doi$$a10.1007/s12274-021-3770-8
000901867 0247_ $$2ISSN$$a1998-0000
000901867 0247_ $$2ISSN$$a1998-0124
000901867 0247_ $$2Handle$$a2128/30723
000901867 0247_ $$2altmetric$$aaltmetric:112752011
000901867 0247_ $$2WOS$$aWOS:000686487500010
000901867 037__ $$aFZJ-2021-03875
000901867 082__ $$a660
000901867 1001_ $$0P:(DE-HGF)0$$aCao, Faqing$$b0
000901867 245__ $$aMechanoadaptive morphing gel electrolyte enables flexible and fast-charging Zn-ion batteries with outstanding dendrite suppression performance
000901867 260__ $$aNew York, NY [u.a.]$$bSpringer$$c2022
000901867 3367_ $$2DRIVER$$aarticle
000901867 3367_ $$2DataCite$$aOutput Types/Journal article
000901867 3367_ $$0PUB:(DE-HGF)16$$2PUB:(DE-HGF)$$aJournal Article$$bjournal$$mjournal$$s1645100769_27455
000901867 3367_ $$2BibTeX$$aARTICLE
000901867 3367_ $$2ORCID$$aJOURNAL_ARTICLE
000901867 3367_ $$00$$2EndNote$$aJournal Article
000901867 520__ $$aThe safe, flexible, and environment-friendly Zn-ion batteries have aroused great interests nowadays. Nevertheless, flagrant Zn dendrite uncontrollably grows in liquid electrolytes due to insufficient surface protection, which severely impedes the future applications of Zn-ion batteries especially at high current densities. Gel electrolytes are emerging to tackle this issue, yet the required high modulus for inhibiting dendrite growth as well as concurrent poor interfacial contact with roughened Zn electrodes are not easily reconcilable to regulate the fragile Zn/Zn2+ interface. Here we demonstrate, such a conflict may be defeated by using a mechanoadaptive cellulose nanofibril-based morphing gel electrolyte (MorphGE), which synergizes bulk compliance for optimizing interfacial contact as well as high modulus for suppressing dendrite formation. Moreover, by anchoring desolvated Zn2+ on cellulose nanofibrils, the side reactions which induce dendrite formation are also significantly reduced. As a result, the MorphGE-based symmetrical Zn-ion battery demonstrated outstanding stability for more than 100 h at the high current density of 10 mA·cm−2 and areal capacity of 10 mA·h·cm−2, and the corresponding Zn-ion battery delivered a prominent specific capacity of 100 mA·h·g−1 for more than 500 cycles at 20 C. The present example of engineering the mechanoadaptivity of gel electrolytes will shed light on a new pathway for designing highly safe and flexible energy storage devices.
000901867 536__ $$0G:(DE-HGF)POF4-6G4$$a6G4 - Jülich Centre for Neutron Research (JCNS) (FZJ) (POF4-6G4)$$cPOF4-6G4$$fPOF IV$$x0
000901867 536__ $$0G:(DE-HGF)POF4-632$$a632 - Materials – Quantum, Complex and Functional Materials (POF4-632)$$cPOF4-632$$fPOF IV$$x1
000901867 588__ $$aDataset connected to CrossRef, Journals: juser.fz-juelich.de
000901867 65027 $$0V:(DE-MLZ)SciArea-180$$2V:(DE-HGF)$$aMaterials Science$$x0
000901867 65017 $$0V:(DE-MLZ)GC-1603-2016$$2V:(DE-HGF)$$aChemical Reactions and Advanced Materials$$x0
000901867 693__ $$0EXP:(DE-MLZ)NOSPEC-20140101$$5EXP:(DE-MLZ)NOSPEC-20140101$$eNo specific instrument$$x0
000901867 7001_ $$0P:(DE-Juel1)151161$$aWu, Baohu$$b1$$ufzj
000901867 7001_ $$0P:(DE-HGF)0$$aLi, Tianyu$$b2
000901867 7001_ $$0P:(DE-HGF)0$$aSun, Shengtong$$b3$$eCorresponding author
000901867 7001_ $$0P:(DE-HGF)0$$aJiao, Yucong$$b4
000901867 7001_ $$0P:(DE-HGF)0$$aWu, Peiyi$$b5$$eCorresponding author
000901867 773__ $$0PERI:(DE-600)2442216-2$$a10.1007/s12274-021-3770-8$$p2030–2039$$tNano research$$v15$$x1998-0000$$y2022
000901867 8564_ $$uhttps://juser.fz-juelich.de/record/901867/files/Cao2022_Article_MechanoadaptiveMorphingGelElec.pdf
000901867 8564_ $$uhttps://juser.fz-juelich.de/record/901867/files/wu_Cao2021-nanoreasearch-last%20draft.pdf$$yPublished on 2021-08-19. Available in OpenAccess from 2022-08-19.
000901867 909CO $$ooai:juser.fz-juelich.de:901867$$pdnbdelivery$$pVDB$$pVDB:MLZ$$pdriver$$popen_access$$popenaire
000901867 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)151161$$aForschungszentrum Jülich$$b1$$kFZJ
000901867 9131_ $$0G:(DE-HGF)POF4-6G4$$1G:(DE-HGF)POF4-6G0$$2G:(DE-HGF)POF4-600$$3G:(DE-HGF)POF4$$4G:(DE-HGF)POF$$aDE-HGF$$bForschungsbereich Materie$$lGroßgeräte: Materie$$vJülich Centre for Neutron Research (JCNS) (FZJ)$$x0
000901867 9131_ $$0G:(DE-HGF)POF4-632$$1G:(DE-HGF)POF4-630$$2G:(DE-HGF)POF4-600$$3G:(DE-HGF)POF4$$4G:(DE-HGF)POF$$aDE-HGF$$bForschungsbereich Materie$$lFrom Matter to Materials and Life$$vMaterials – Quantum, Complex and Functional Materials$$x1
000901867 9141_ $$y2022
000901867 915__ $$0StatID:(DE-HGF)0530$$2StatID$$aEmbargoed OpenAccess
000901867 915__ $$0StatID:(DE-HGF)0113$$2StatID$$aWoS$$bScience Citation Index Expanded$$d2021-01-30
000901867 915__ $$0StatID:(DE-HGF)3002$$2StatID$$aDEAL Springer$$d2021-01-30$$wger
000901867 915__ $$0StatID:(DE-HGF)0160$$2StatID$$aDBCoverage$$bEssential Science Indicators$$d2021-01-30
000901867 915__ $$0StatID:(DE-HGF)0100$$2StatID$$aJCR$$bNANO RES : 2021$$d2022-11-11
000901867 915__ $$0StatID:(DE-HGF)0200$$2StatID$$aDBCoverage$$bSCOPUS$$d2022-11-11
000901867 915__ $$0StatID:(DE-HGF)0300$$2StatID$$aDBCoverage$$bMedline$$d2022-11-11
000901867 915__ $$0StatID:(DE-HGF)0199$$2StatID$$aDBCoverage$$bClarivate Analytics Master Journal List$$d2022-11-11
000901867 915__ $$0StatID:(DE-HGF)1160$$2StatID$$aDBCoverage$$bCurrent Contents - Engineering, Computing and Technology$$d2022-11-11
000901867 915__ $$0StatID:(DE-HGF)0150$$2StatID$$aDBCoverage$$bWeb of Science Core Collection$$d2022-11-11
000901867 915__ $$0StatID:(DE-HGF)1150$$2StatID$$aDBCoverage$$bCurrent Contents - Physical, Chemical and Earth Sciences$$d2022-11-11
000901867 915__ $$0StatID:(DE-HGF)9910$$2StatID$$aIF >= 10$$bNANO RES : 2021$$d2022-11-11
000901867 920__ $$lyes
000901867 9201_ $$0I:(DE-Juel1)JCNS-4-20201012$$kJCNS-4$$lJCNS-4$$x0
000901867 9201_ $$0I:(DE-Juel1)JCNS-FRM-II-20110218$$kJCNS-FRM-II$$lJCNS-FRM-II$$x1
000901867 9201_ $$0I:(DE-Juel1)JCNS-1-20110106$$kJCNS-1$$lNeutronenstreuung$$x2
000901867 9201_ $$0I:(DE-588b)4597118-3$$kMLZ$$lHeinz Maier-Leibnitz Zentrum$$x3
000901867 980__ $$ajournal
000901867 980__ $$aVDB
000901867 980__ $$aUNRESTRICTED
000901867 980__ $$aI:(DE-Juel1)JCNS-4-20201012
000901867 980__ $$aI:(DE-Juel1)JCNS-FRM-II-20110218
000901867 980__ $$aI:(DE-Juel1)JCNS-1-20110106
000901867 980__ $$aI:(DE-588b)4597118-3
000901867 9801_ $$aFullTexts