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000901868 1001_ $$0P:(DE-HGF)0$$aZhang, Wei$$b0
000901868 245__ $$aSkin-like mechanoresponsive self-healing ionic elastomer from supramolecular zwitterionic network
000901868 260__ $$a[London]$$bNature Publishing Group UK$$c2021
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000901868 520__ $$aStretchable ionic skins are intriguing in mimicking the versatile sensations of natural skins. However, for their applications in advanced electronics, good elastic recovery, self-healing, and more importantly, skin-like nonlinear mechanoresponse (strain-stiffening) are essential but can be rarely met in one material. Here we demonstrate a robust proton-conductive ionic skin design via introducing an entropy-driven supramolecular zwitterionic reorganizable network to the hydrogen-bonded polycarboxylic acid network. The design allows two dynamic networks with distinct interacting strength to sequentially debond with stretch, and the conflict among elasticity, self-healing, and strain-stiffening can be thus defeated. The representative polyacrylic acid/betaine elastomer exhibits high stretchability (1600% elongation), immense strain-stiffening (24-fold modulus enhancement), ~100% self-healing, excellent elasticity (97.9 ± 1.1% recovery ratio, <14% hysteresis), high transparency (99.7 ± 0.1%), moisture-preserving, anti-freezing (elastic at −40 °C), water reprocessibility, as well as easy-to-peel adhesion. The combined advantages make the present ionic elastomer very promising in wearable iontronic sensors for human-machine interfacing
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000901868 65017 $$0V:(DE-MLZ)GC-1602-2016$$2V:(DE-HGF)$$aPolymers, Soft Nano Particles and  Proteins$$x0
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000901868 7001_ $$0P:(DE-Juel1)151161$$aWu, Baohu$$b1$$ufzj
000901868 7001_ $$00000-0001-7471-686X$$aSun, Shengtong$$b2$$eCorresponding author
000901868 7001_ $$00000-0001-7235-210X$$aWu, Peiyi$$b3$$eCorresponding author
000901868 773__ $$0PERI:(DE-600)2553671-0$$a10.1038/s41467-021-24382-4$$gVol. 12, no. 1, p. 4082$$n1$$p4082$$tNature Communications$$v12$$x2041-1723$$y2021
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