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| Hauptseite > Publikationsdatenbank > Skin-like mechanoresponsive self-healing ionic elastomer from supramolecular zwitterionic network > print |
| Hauptseite > Publikationsdatenbank > Skin-like mechanoresponsive self-healing ionic elastomer from supramolecular zwitterionic network > print |
| 001 | 901868 | ||
| 005 | 20211130111104.0 | ||
| 024 | 7 | _ | |a 10.1038/s41467-021-24382-4 |2 doi |
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| 100 | 1 | _ | |a Zhang, Wei |0 P:(DE-HGF)0 |b 0 |
| 245 | _ | _ | |a Skin-like mechanoresponsive self-healing ionic elastomer from supramolecular zwitterionic network |
| 260 | _ | _ | |a [London] |c 2021 |b Nature Publishing Group UK |
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| 520 | _ | _ | |a Stretchable ionic skins are intriguing in mimicking the versatile sensations of natural skins. However, for their applications in advanced electronics, good elastic recovery, self-healing, and more importantly, skin-like nonlinear mechanoresponse (strain-stiffening) are essential but can be rarely met in one material. Here we demonstrate a robust proton-conductive ionic skin design via introducing an entropy-driven supramolecular zwitterionic reorganizable network to the hydrogen-bonded polycarboxylic acid network. The design allows two dynamic networks with distinct interacting strength to sequentially debond with stretch, and the conflict among elasticity, self-healing, and strain-stiffening can be thus defeated. The representative polyacrylic acid/betaine elastomer exhibits high stretchability (1600% elongation), immense strain-stiffening (24-fold modulus enhancement), ~100% self-healing, excellent elasticity (97.9 ± 1.1% recovery ratio, <14% hysteresis), high transparency (99.7 ± 0.1%), moisture-preserving, anti-freezing (elastic at −40 °C), water reprocessibility, as well as easy-to-peel adhesion. The combined advantages make the present ionic elastomer very promising in wearable iontronic sensors for human-machine interfacing |
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| 700 | 1 | _ | |a Sun, Shengtong |0 0000-0001-7471-686X |b 2 |e Corresponding author |
| 700 | 1 | _ | |a Wu, Peiyi |0 0000-0001-7235-210X |b 3 |e Corresponding author |
| 773 | _ | _ | |a 10.1038/s41467-021-24382-4 |g Vol. 12, no. 1, p. 4082 |0 PERI:(DE-600)2553671-0 |n 1 |p 4082 |t Nature Communications |v 12 |y 2021 |x 2041-1723 |
| 856 | 4 | _ | |u https://juser.fz-juelich.de/record/901868/files/3.s41467-021-24382-4.pdf |y OpenAccess |
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