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@ARTICLE{Lei:901871,
author = {Lei, Zhouyue and Wu, Baohu and Wu, Peiyi},
title = {{H}ierarchical {N}etwork-{A}ugmented {H}ydroglasses for
{B}roadband {L}ight {M}anagement},
journal = {Research},
volume = {2021},
issn = {2639-5274},
address = {[Beijing]},
publisher = {China Association for Science and Technology},
reportid = {FZJ-2021-03879},
pages = {Article ID 4515164},
year = {2021},
abstract = {Light management is essential for military stealth, optical
information communication, and energy-efficient buildings.
However, current light management materials face challenges
of limited optical modulation range and poor mechanical
properties. Herein, we report a locally confined
polymerization (LCP) approach to develop hierarchical
network-augmented hydroglasses (HNAH) based on
poly(methacrylic acid) for broadband light management as
well as mechanical enhancement. The dynamic geometry of the
networks ranging from nano- to micro-scale enables to manage
the light wavelength over three orders of magnitude, from
the ultraviolet (UV) to infrared (IR) band, and reversibly
switches transmittance in the visible region. A smart
hydroglass window is developed with elasticity, outstanding
robustness, self-healing, notch resistance, biosafety by
blocking UV radiation, and high solar energy shielding
efficacy with a temperature drop of 13°C. Compared to
current inorganic glasses and Plexiglas, the hydroglass not
only is a promising and versatile candidate but also
provides novel insights into the molecular and structural
design of broadband light management and optimized
mechanical properties.},
cin = {JCNS-4 / JCNS-1 / JCNS-FRM-II / MLZ},
ddc = {600},
cid = {I:(DE-Juel1)JCNS-4-20201012 / I:(DE-Juel1)JCNS-1-20110106 /
I:(DE-Juel1)JCNS-FRM-II-20110218 / I:(DE-588b)4597118-3},
pnm = {6G4 - Jülich Centre for Neutron Research (JCNS) (FZJ)
(POF4-6G4) / 632 - Materials – Quantum, Complex and
Functional Materials (POF4-632)},
pid = {G:(DE-HGF)POF4-6G4 / G:(DE-HGF)POF4-632},
experiment = {EXP:(DE-MLZ)KWS3-20140101},
typ = {PUB:(DE-HGF)16},
pubmed = {33623918},
UT = {WOS:000610827400001},
doi = {10.34133/2021/4515164},
url = {https://juser.fz-juelich.de/record/901871},
}