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100 1 _ |a Schick, Daniel
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245 _ _ |a Laser-driven resonant magnetic soft-x-ray scattering for probing ultrafast antiferromagnetic and structural dynamics
260 _ _ |a Washington, DC
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520 _ _ |a Time-resolved resonant magnetic scattering in the soft-x-ray range is a powerful tool for accessing the spatially resolved and element-specific spin dynamics in magnetic materials. So far, the application of this photon-demanding technique was limited to large-scale facilities. However, upgrades to diffraction-limited storage rings supporting only x-ray pulses beyond 100 ps, and the shift of x-ray free-electron lasers toward attosecond pulses aggravate the competition for beamtime in the picosecond time window, which is of utmost relevance for magnetism research. Here we present the development of a lab-based instrument providing sufficient photon flux up to 1.5 keV photon energy covering the soft-x-ray resonances of transition and rare-earth metal atoms. Our setup features the mandatory tunability in energy and reciprocal space in combination with sub-10 ps temporal resolution, exploiting the broadband emission of a laser-driven plasma x-ray source, which is monochromatized to about 1 eV bandwidth by a reflection zone plate. We benchmark our approach against accelerator-based soft-x-ray sources by simultaneously probing the laser-induced magnetic and structural dynamics from an antiferromagnetically coupled Fe/Cr superlattice. Our development lays the foundation for laser-driven resonant scattering experiments to study ultrafast ordering phenomena of charges, spins, and orbitals.
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700 1 _ |a Borchert, Martin
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700 1 _ |a Braenzel, Julia
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700 1 _ |a Stiel, Holger
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700 1 _ |a Tümmler, Johannes
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700 1 _ |a Bürgler, Daniel E.
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700 1 _ |a Firsov, Alexander
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700 1 _ |a von Korff Schmising, Clemens
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700 1 _ |a Pfau, Bastian
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700 1 _ |a Eisebitt, Stefan
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773 _ _ |a 10.1364/OPTICA.435522
|g Vol. 8, no. 9, p. 1237 -
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