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@ARTICLE{Wang:902192,
author = {Wang, Yaping and Sergeev, Dmitry and Yazhenskikh, Elena and
Pillai, Rishi and Müller, Michael and Naumenko, Dmitry},
title = {{E}xperimental study coupled with thermodynamic assessment
of the {N}i{SO}4–{K}2{SO}4 quasi binary system},
journal = {Calphad},
volume = {74},
issn = {0364-5916},
address = {Amsterdam [u.a.]},
publisher = {Elsevier Science},
reportid = {FZJ-2021-04089},
pages = {102328 -},
year = {2021},
abstract = {Thermodynamic properties of the NiSO4–K2SO4 system play
significant roles in various applications, e. g. in gas
turbine components. In these components, Ni-base superalloys
and coatings often suffer from the so-called hot corrosion
induced by alkali sulphate deposits. In the present work,
the phase equilibria in the system NiSO4–K2SO4 were
experimentally determined for the first time using
differential thermal analysis (DTA), dilatometry (DiL) and
X-ray diffraction method (XRD). Two eutectic points and two
stoichiometric compounds, K2Ni2(SO4)3 and K2Ni(SO4)2, were
found in this system. The temperature and composition of the
lower eutectic were determined to be 642 °C and 40 $mol.\%$
NiSO4, respectively. Another eutectic between NiSO4 and
K2Ni2(SO4)3 was found at 819 °C, and the corresponding
composition is around 75 $mol.\%$ NiSO4 and 25 mol. $\%$
K2SO4. Based on the obtained experimental data, the
NiSO4–K2SO4 system was thermodynamically assessed using
the CALPHAD methodology. The modified associate species
model was used for the description of the liquid phase.
Using the optimized dataset, the calculated phase diagram
showed a good agreement with the experimental results. This
dataset extends the previously developed general sulphate
database including alkali- and alkaline-earth sulphates
(CaSO4–MgSO4–Na2SO4–K2SO4) with the addition of
NiSO4.},
cin = {IEK-2},
ddc = {540},
cid = {I:(DE-Juel1)IEK-2-20101013},
pnm = {1221 - Fundamentals and Materials (POF4-122)},
pid = {G:(DE-HGF)POF4-1221},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000685310300005},
doi = {10.1016/j.calphad.2021.102328},
url = {https://juser.fz-juelich.de/record/902192},
}