Gast ::
| Hauptseite > Publikationsdatenbank > Effect of NOx on 1,3,5-trimethylbenzene (TMB) oxidation product distribution and particle formation > print |
| Hauptseite > Publikationsdatenbank > Effect of NOx on 1,3,5-trimethylbenzene (TMB) oxidation product distribution and particle formation > print |
| 001 | 902269 | ||
| 005 | 20240712101023.0 | ||
| 024 | 7 | _ | |a 10.5194/acp-19-15073-2019 |2 doi |
| 024 | 7 | _ | |a 1680-7316 |2 ISSN |
| 024 | 7 | _ | |a 1680-7324 |2 ISSN |
| 024 | 7 | _ | |a 2128/28922 |2 Handle |
| 024 | 7 | _ | |a altmetric:72722444 |2 altmetric |
| 024 | 7 | _ | |a WOS:000502996800002 |2 WOS |
| 037 | _ | _ | |a FZJ-2021-04132 |
| 082 | _ | _ | |a 550 |
| 100 | 1 | _ | |a Tsiligiannis, Epameinondas |0 0000-0002-5100-0858 |b 0 |
| 245 | _ | _ | |a Effect of NOx on 1,3,5-trimethylbenzene (TMB) oxidation product distribution and particle formation |
| 260 | _ | _ | |a Katlenburg-Lindau |c 2019 |b EGU |
| 336 | 7 | _ | |a article |2 DRIVER |
| 336 | 7 | _ | |a Output Types/Journal article |2 DataCite |
| 336 | 7 | _ | |a Journal Article |b journal |m journal |0 PUB:(DE-HGF)16 |s 1636368327_22372 |2 PUB:(DE-HGF) |
| 336 | 7 | _ | |a ARTICLE |2 BibTeX |
| 336 | 7 | _ | |a JOURNAL_ARTICLE |2 ORCID |
| 336 | 7 | _ | |a Journal Article |0 0 |2 EndNote |
| 520 | _ | _ | |a Secondary organic aerosol (SOA) represents a significant fraction of the tropospheric aerosol and its precursors are volatile organic compounds (VOCs). Anthropogenic VOCs (AVOC) dominate the VOC budget in many urban areas with 1,3,5-trimethylbenzene (TMB) being among the most reactive aromatic AVOCs. TMB formed highly oxygenated organic molecules (HOMs) in an NOx-free environment, which could contribute to new particle formation (NPF) depending on oxidation conditions where elevated OH oxidation enhanced particle formation. The experiments were performed in an oxidation flow reactor, the Go:PAM unit, under controlled OH oxidation conditions. By addition of NOx to the system we investigated the effect of NOx on particle formation and on the product distribution. We show that the formation of HOMs, and especially HOM accretion products, strongly varies with NOx conditions. We observe a suppression of HOM and particle formation with increasing NOx/ΔTMB ratio and an increase in the formation of organonitrates (ONs) mostly at the expense of HOM accretion products. We propose reaction mechanisms and pathways that explain the formation and observed product distributions with respect to oxidation conditions. We hypothesise that, based on our findings from TMB oxidation studies, aromatic AVOCs may not contribute significantly to NPF under typical NOx/AVOC conditions found in urban atmospheres. |
| 536 | _ | _ | |a 2111 - Air Quality (POF4-211) |0 G:(DE-HGF)POF4-2111 |c POF4-211 |f POF IV |x 0 |
| 588 | _ | _ | |a Dataset connected to CrossRef, Journals: juser.fz-juelich.de |
| 700 | 1 | _ | |a Hammes, Julia |0 0000-0003-2333-2596 |b 1 |
| 700 | 1 | _ | |a Salvador, Christian Mark |0 0000-0002-8328-7777 |b 2 |
| 700 | 1 | _ | |a Mentel, Thomas F. |0 P:(DE-Juel1)16346 |b 3 |
| 700 | 1 | _ | |a Hallquist, Mattias |0 P:(DE-HGF)0 |b 4 |e Corresponding author |
| 773 | _ | _ | |a 10.5194/acp-19-15073-2019 |g Vol. 19, no. 23, p. 15073 - 15086 |0 PERI:(DE-600)2069847-1 |n 23 |p 15073 - 15086 |t Atmospheric chemistry and physics |v 19 |y 2019 |x 1680-7324 |
| 856 | 4 | _ | |u https://juser.fz-juelich.de/record/902269/files/acp-19-15073-2019.pdf |y OpenAccess |
| 909 | C | O | |o oai:juser.fz-juelich.de:902269 |p openaire |p open_access |p VDB |p driver |p dnbdelivery |
| 910 | 1 | _ | |a Forschungszentrum Jülich |0 I:(DE-588b)5008462-8 |k FZJ |b 3 |6 P:(DE-Juel1)16346 |
| 913 | 1 | _ | |a DE-HGF |b Forschungsbereich Erde und Umwelt |l Erde im Wandel – Unsere Zukunft nachhaltig gestalten |1 G:(DE-HGF)POF4-210 |0 G:(DE-HGF)POF4-211 |3 G:(DE-HGF)POF4 |2 G:(DE-HGF)POF4-200 |4 G:(DE-HGF)POF |v Die Atmosphäre im globalen Wandel |9 G:(DE-HGF)POF4-2111 |x 0 |
| 914 | 1 | _ | |y 2021 |
| 915 | _ | _ | |a DBCoverage |0 StatID:(DE-HGF)0200 |2 StatID |b SCOPUS |d 2021-02-02 |
| 915 | _ | _ | |a DBCoverage |0 StatID:(DE-HGF)0160 |2 StatID |b Essential Science Indicators |d 2021-02-02 |
| 915 | _ | _ | |a Creative Commons Attribution CC BY 4.0 |0 LIC:(DE-HGF)CCBY4 |2 HGFVOC |
| 915 | _ | _ | |a DBCoverage |0 StatID:(DE-HGF)1150 |2 StatID |b Current Contents - Physical, Chemical and Earth Sciences |d 2021-02-02 |
| 915 | _ | _ | |a IF >= 5 |0 StatID:(DE-HGF)9905 |2 StatID |b ATMOS CHEM PHYS : 2019 |d 2021-02-02 |
| 915 | _ | _ | |a DBCoverage |0 StatID:(DE-HGF)0501 |2 StatID |b DOAJ Seal |d 2021-02-02 |
| 915 | _ | _ | |a DBCoverage |0 StatID:(DE-HGF)0500 |2 StatID |b DOAJ |d 2021-02-02 |
| 915 | _ | _ | |a WoS |0 StatID:(DE-HGF)0113 |2 StatID |b Science Citation Index Expanded |d 2021-02-02 |
| 915 | _ | _ | |a Fees |0 StatID:(DE-HGF)0700 |2 StatID |d 2021-02-02 |
| 915 | _ | _ | |a DBCoverage |0 StatID:(DE-HGF)0150 |2 StatID |b Web of Science Core Collection |d 2021-02-02 |
| 915 | _ | _ | |a OpenAccess |0 StatID:(DE-HGF)0510 |2 StatID |
| 915 | _ | _ | |a Peer Review |0 StatID:(DE-HGF)0030 |2 StatID |b DOAJ : Peer review |d 2021-02-02 |
| 915 | _ | _ | |a Article Processing Charges |0 StatID:(DE-HGF)0561 |2 StatID |d 2021-02-02 |
| 915 | _ | _ | |a JCR |0 StatID:(DE-HGF)0100 |2 StatID |b ATMOS CHEM PHYS : 2019 |d 2021-02-02 |
| 915 | _ | _ | |a DBCoverage |0 StatID:(DE-HGF)0300 |2 StatID |b Medline |d 2021-02-02 |
| 915 | _ | _ | |a DBCoverage |0 StatID:(DE-HGF)0199 |2 StatID |b Clarivate Analytics Master Journal List |d 2021-02-02 |
| 920 | 1 | _ | |0 I:(DE-Juel1)IEK-8-20101013 |k IEK-8 |l Troposphäre |x 0 |
| 980 | 1 | _ | |a FullTexts |
| 980 | _ | _ | |a journal |
| 980 | _ | _ | |a VDB |
| 980 | _ | _ | |a UNRESTRICTED |
| 980 | _ | _ | |a I:(DE-Juel1)IEK-8-20101013 |
| 981 | _ | _ | |a I:(DE-Juel1)ICE-3-20101013 |
| Library | Collection | CLSMajor | CLSMinor | Language | Author |
|---|