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| 001 | 902326 | ||
| 005 | 20240712113111.0 | ||
| 024 | 7 | _ | |a 10.1016/j.ensm.2021.10.017 |2 doi |
| 024 | 7 | _ | |a 2405-8289 |2 ISSN |
| 024 | 7 | _ | |a 2405-8297 |2 ISSN |
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| 037 | _ | _ | |a FZJ-2021-04183 |
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| 100 | 1 | _ | |a Shaji, Ishamol |0 P:(DE-Juel1)174187 |b 0 |
| 245 | _ | _ | |a Multisalt chemistry in ion transport and interface of lithium metal polymer batteries |
| 260 | _ | _ | |a Amsterdam |c 2022 |b Elsevier |
| 336 | 7 | _ | |a article |2 DRIVER |
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| 520 | _ | _ | |a Solvent-free solid-state polymer electrolytes (SPE) that go beyond the barriers like intrinsic low ionic conductivity, slow ion dynamics, and unstable electrode-electrolyte interphase will be fundamental for realizing the next generation of safe and high-performance lithium metal batteries. Hereby, cross-linked solid polymer electrolyte (XSPE) networks based on multisalt chemistry are synthesized using photopolymerization reaction, which outshine the conventional single salt-based XSPEs. By introducing the multisalt chemistry, an enhanced Li+ ion transport (ionic conductivity and short residence time) via anion mediated transfer (AMT) and improved interfacial characteristics (e.g., stable Li|electrolyte interphase, smooth Li-deposition) are demonstrated. Furthermore, a three-times increase in Li+ ion transference number and nearly one order of magnitude increment in diffusion coefficient are achieved. Using theoretical calculations, we propose an AMT-based ion conduction pathway in multisalt-based XSPEs. Besides, the superior electrochemical performance of multisalt-based XSPEs compared to single salt-based polymer electrolytes in Li-metal polymer batteries (LMPB) using C-LiFePO4 and LiNi0.8Co0.15Al0.05O2 cathodes are successfully demonstrated. |
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| 700 | 1 | _ | |a Diddens, Diddo |0 P:(DE-Juel1)169877 |b 1 |
| 700 | 1 | _ | |a Ehteshami, Niloofar |0 P:(DE-Juel1)168592 |b 2 |
| 700 | 1 | _ | |a Winter, Martin |0 P:(DE-Juel1)166130 |b 3 |e Corresponding author |
| 700 | 1 | _ | |a Nair, Jijeesh Ravi |0 P:(DE-Juel1)171863 |b 4 |e Corresponding author |
| 773 | _ | _ | |a 10.1016/j.ensm.2021.10.017 |g Vol. 44, p. 263 - 277 |0 PERI:(DE-600)2841602-8 |p 263 - 277 |t Energy storage materials |v 44 |y 2022 |x 2405-8297 |
| 856 | 4 | _ | |u https://juser.fz-juelich.de/record/902326/files/Journal%20article.pdf |y Restricted |
| 856 | 4 | _ | |y Published on 2021-10-14. Available in OpenAccess from 2022-10-14. |u https://juser.fz-juelich.de/record/902326/files/Accepted%20manuscript.pdf |
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