000902337 001__ 902337
000902337 005__ 20240715202022.0
000902337 0247_ $$2doi$$a10.1016/j.atmosenv.2021.118842
000902337 0247_ $$2ISSN$$a0004-6981
000902337 0247_ $$2ISSN$$a1352-2310
000902337 0247_ $$2ISSN$$a1873-2844
000902337 0247_ $$2ISSN$$a(BIS
000902337 0247_ $$2ISSN$$a1989)
000902337 0247_ $$2ISSN$$a1878-2442
000902337 0247_ $$2Handle$$a2128/29186
000902337 0247_ $$2WOS$$aWOS:000780429300001
000902337 037__ $$aFZJ-2021-04186
000902337 082__ $$a690
000902337 1001_ $$0P:(DE-Juel1)180665$$aKhundadze, Nana$$b0$$ufzj
000902337 245__ $$aBenchmarking source specific isotopic ratios of levoglucosan to better constrain the contribution of domestic heating to the air pollution
000902337 260__ $$aAmsterdam [u.a.]$$bElsevier Science$$c2022
000902337 3367_ $$2DRIVER$$aarticle
000902337 3367_ $$2DataCite$$aOutput Types/Journal article
000902337 3367_ $$0PUB:(DE-HGF)16$$2PUB:(DE-HGF)$$aJournal Article$$bjournal$$mjournal$$s1721024194_11706
000902337 3367_ $$2BibTeX$$aARTICLE
000902337 3367_ $$2ORCID$$aJOURNAL_ARTICLE
000902337 3367_ $$00$$2EndNote$$aJournal Article
000902337 520__ $$aWe report source specific isotope ratios of levoglucosan, the specific biomass burning tracer, in aerosol particle from the combustion of selected woods used for domestic heating in Europe, of coals containing cellulose (lignites) as well as of corn, a C4 plant. Here, we combine compound specific δ13C measurements of levoglucosan with total carbon δ13C of parent materials, to assess isotopic fractionations due to biosynthetic pathways or combustion processes. Levoglucosan formed during the combustion of cellulose from coals shows with δ13C of −21.1‰ and −18.6‰ a moderate enrichment in the heavier isotope compared to the C3 plant samples. Contrarily, observed levoglucosan isotope ratios of −25.0 to −21.5‰ for C3 plant samples are significantly lower than for the C4 plant sample (−12.4‰), as expected from the stronger 13C discrimination during the carbon fixation process by C3 compared to C4 plants. Overall, the C4 plant sample shows a 13C enrichment in all bulk measurements, on average by 12.2‰, 14.2‰ and 14.2‰ for total carbon (TC) in aerosol particle, whole plant/coal material and cellulose samples, respectively. Further, δ13C measurements of levoglucosan and TC of biomass burning aerosol particles, bulk plant/coal and cellulose in C3 plant samples agree well with the published observations. The combined levoglucosan/TC isotopic analyses can be used to differentiate among C3/coal/C4 origin of the smoke emissions from the cellulose-containing-fuel combustion. Noticeably, there is a consistent δ13C offset between C3 plant material and levoglucosan, which allows deriving emission levoglucosan isotope ratios when the combusted plant types are known.
000902337 536__ $$0G:(DE-HGF)POF4-2111$$a2111 - Air Quality (POF4-211)$$cPOF4-211$$fPOF IV$$x0
000902337 536__ $$0G:(DE-HGF)POF4-2173$$a2173 - Agro-biogeosystems: controls, feedbacks and impact (POF4-217)$$cPOF4-217$$fPOF IV$$x1
000902337 588__ $$aDataset connected to CrossRef, Journals: juser.fz-juelich.de
000902337 7001_ $$0P:(DE-Juel1)167368$$aKüppers, Christoph$$b1$$ufzj
000902337 7001_ $$0P:(DE-Juel1)129212$$aKammer, Beatrix$$b2$$ufzj
000902337 7001_ $$00000-0002-3105-8059$$aGarbaras, Andrius$$b3
000902337 7001_ $$0P:(DE-HGF)0$$aMasalaite, Agne$$b4
000902337 7001_ $$0P:(DE-Juel1)129557$$aWissel, Holger$$b5$$ufzj
000902337 7001_ $$0P:(DE-Juel1)129567$$aLücke, Andreas$$b6$$ufzj
000902337 7001_ $$0P:(DE-HGF)0$$aChankvetadze, Bezhan$$b7
000902337 7001_ $$0P:(DE-Juel1)172931$$aRudolph, Jochen$$b8
000902337 7001_ $$0P:(DE-Juel1)4528$$aKiendler-Scharr, Astrid$$b9$$ufzj
000902337 7001_ $$0P:(DE-Juel1)6110$$aGensch, Iulia$$b10$$eCorresponding author
000902337 773__ $$0PERI:(DE-600)1499889-0$$a10.1016/j.atmosenv.2021.118842$$gp. 118842 -$$p118842$$tAtmospheric environment$$v268$$x0004-6981$$y2022
000902337 8564_ $$uhttps://juser.fz-juelich.de/record/902337/files/Invoice_OAD0000159405.pdf
000902337 8564_ $$uhttps://juser.fz-juelich.de/record/902337/files/Invoice_W1586390.pdf
000902337 8564_ $$uhttps://juser.fz-juelich.de/record/902337/files/1-s2.0-S1352231021006646-main.pdf$$yOpenAccess
000902337 8767_ $$8OAD0000159405$$92021-11-08$$d2021-11-15$$eHybrid-OA$$jZahlung erfolgt$$zBelegnr.: 1200173350
000902337 8767_ $$8W1586390$$92021-11-15$$d2021-11-19$$eColour charges$$jZahlung erfolgt$$zBelegnr.: 1200173534
000902337 909CO $$ooai:juser.fz-juelich.de:902337$$popenaire$$pdnbdelivery$$popenCost$$pVDB$$pdriver$$pOpenAPC$$popen_access
000902337 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)180665$$aForschungszentrum Jülich$$b0$$kFZJ
000902337 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)167368$$aForschungszentrum Jülich$$b1$$kFZJ
000902337 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)129212$$aForschungszentrum Jülich$$b2$$kFZJ
000902337 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)129557$$aForschungszentrum Jülich$$b5$$kFZJ
000902337 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)129567$$aForschungszentrum Jülich$$b6$$kFZJ
000902337 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)4528$$aForschungszentrum Jülich$$b9$$kFZJ
000902337 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)6110$$aForschungszentrum Jülich$$b10$$kFZJ
000902337 9131_ $$0G:(DE-HGF)POF4-211$$1G:(DE-HGF)POF4-210$$2G:(DE-HGF)POF4-200$$3G:(DE-HGF)POF4$$4G:(DE-HGF)POF$$9G:(DE-HGF)POF4-2111$$aDE-HGF$$bForschungsbereich Erde und Umwelt$$lErde im Wandel – Unsere Zukunft nachhaltig gestalten$$vDie Atmosphäre im globalen Wandel$$x0
000902337 9131_ $$0G:(DE-HGF)POF4-217$$1G:(DE-HGF)POF4-210$$2G:(DE-HGF)POF4-200$$3G:(DE-HGF)POF4$$4G:(DE-HGF)POF$$9G:(DE-HGF)POF4-2173$$aDE-HGF$$bForschungsbereich Erde und Umwelt$$lErde im Wandel – Unsere Zukunft nachhaltig gestalten$$vFür eine nachhaltige Bio-Ökonomie – von Ressourcen zu Produkten$$x1
000902337 9141_ $$y2022
000902337 915__ $$0StatID:(DE-HGF)0160$$2StatID$$aDBCoverage$$bEssential Science Indicators$$d2021-01-29
000902337 915__ $$0StatID:(DE-HGF)1190$$2StatID$$aDBCoverage$$bBiological Abstracts$$d2021-01-29
000902337 915__ $$0StatID:(DE-HGF)0113$$2StatID$$aWoS$$bScience Citation Index Expanded$$d2021-01-29
000902337 915__ $$0StatID:(DE-HGF)0510$$2StatID$$aOpenAccess
000902337 915__ $$0LIC:(DE-HGF)CCBY4$$2HGFVOC$$aCreative Commons Attribution CC BY 4.0
000902337 915__ $$0StatID:(DE-HGF)0420$$2StatID$$aNationallizenz$$d2022-11-19$$wger
000902337 915__ $$0StatID:(DE-HGF)0200$$2StatID$$aDBCoverage$$bSCOPUS$$d2022-11-19
000902337 915__ $$0StatID:(DE-HGF)0300$$2StatID$$aDBCoverage$$bMedline$$d2022-11-19
000902337 915__ $$0StatID:(DE-HGF)0100$$2StatID$$aJCR$$bATMOS ENVIRON : 2021$$d2022-11-19
000902337 915__ $$0StatID:(DE-HGF)0600$$2StatID$$aDBCoverage$$bEbsco Academic Search$$d2022-11-19
000902337 915__ $$0StatID:(DE-HGF)0030$$2StatID$$aPeer Review$$bASC$$d2022-11-19
000902337 915__ $$0StatID:(DE-HGF)0199$$2StatID$$aDBCoverage$$bClarivate Analytics Master Journal List$$d2022-11-19
000902337 915__ $$0StatID:(DE-HGF)0150$$2StatID$$aDBCoverage$$bWeb of Science Core Collection$$d2022-11-19
000902337 915__ $$0StatID:(DE-HGF)1050$$2StatID$$aDBCoverage$$bBIOSIS Previews$$d2022-11-19
000902337 915__ $$0StatID:(DE-HGF)1060$$2StatID$$aDBCoverage$$bCurrent Contents - Agriculture, Biology and Environmental Sciences$$d2022-11-19
000902337 915__ $$0StatID:(DE-HGF)1150$$2StatID$$aDBCoverage$$bCurrent Contents - Physical, Chemical and Earth Sciences$$d2022-11-19
000902337 915__ $$0StatID:(DE-HGF)9905$$2StatID$$aIF >= 5$$bATMOS ENVIRON : 2021$$d2022-11-19
000902337 9201_ $$0I:(DE-Juel1)IEK-8-20101013$$kIEK-8$$lTroposphäre$$x0
000902337 9201_ $$0I:(DE-Juel1)IBG-3-20101118$$kIBG-3$$lAgrosphäre$$x1
000902337 980__ $$ajournal
000902337 980__ $$aVDB
000902337 980__ $$aI:(DE-Juel1)IEK-8-20101013
000902337 980__ $$aI:(DE-Juel1)IBG-3-20101118
000902337 980__ $$aAPC
000902337 980__ $$aUNRESTRICTED
000902337 9801_ $$aAPC
000902337 9801_ $$aFullTexts
000902337 981__ $$aI:(DE-Juel1)ICE-3-20101013