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| Hauptseite > Publikationsdatenbank > Fabrication of multi-layered structures for proton conducting ceramic cells > print |
| Hauptseite > Publikationsdatenbank > Fabrication of multi-layered structures for proton conducting ceramic cells > print |
| 001 | 902340 | ||
| 005 | 20240711085638.0 | ||
| 024 | 7 | _ | |a 10.1039/D1TA05240C |2 doi |
| 024 | 7 | _ | |a 2050-7488 |2 ISSN |
| 024 | 7 | _ | |a 2050-7496 |2 ISSN |
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| 037 | _ | _ | |a FZJ-2021-04189 |
| 082 | _ | _ | |a 530 |
| 100 | 1 | _ | |a Deibert, Wendelin |0 P:(DE-Juel1)144923 |b 0 |e Corresponding author |u fzj |
| 245 | _ | _ | |a Fabrication of multi-layered structures for proton conducting ceramic cells |
| 260 | _ | _ | |a London [u.a.] |c 2022 |b RSC |
| 336 | 7 | _ | |a article |2 DRIVER |
| 336 | 7 | _ | |a Output Types/Journal article |2 DataCite |
| 336 | 7 | _ | |a Journal Article |b journal |m journal |0 PUB:(DE-HGF)16 |s 1644830964_13686 |2 PUB:(DE-HGF) |
| 336 | 7 | _ | |a ARTICLE |2 BibTeX |
| 336 | 7 | _ | |a JOURNAL_ARTICLE |2 ORCID |
| 336 | 7 | _ | |a Journal Article |0 0 |2 EndNote |
| 520 | _ | _ | |a Protonic ceramic fuel cells offer a high potential to produce electrical energy in a very efficient way. The performance of such a device among others is highly dependent on the electrolyte material and its thickness. Therefore, multilayer structures are used to reduce the electrolyte thickness down to 10–20 μm, supported by a much thicker porous anode. In this work sequential tape-casting is used to fabricate half-cells consisting of a BZCY electrolyte and a BZCY/NiO support which also serves as the anode layer. The starting powders are characterised as well as the thermal behaviour of the half-cells during heat treatment. Sintering experiments show that a temperature of T ≥ 1450 °C is needed to achieve the desired microstructure. After that a scale-up approach to a size of the half-cells of about 25 cm2 is shown. The influence of the processing temperature on the microstructure is shown by detailed XRD and SEM studies. The formation of a BaY2NiO5 transient liquid phase during the heat treatment of the cells is clearly demonstrated. Finally, the proton conductivity of the tape-cast cells shows competitive values of σ = 0.003 S cm−1 at 600 °C with the advantage of an industrially proven and up-scalable manufacturing technique. |
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| 700 | 1 | _ | |a Ivanova, Mariya E. |0 P:(DE-Juel1)129617 |b 1 |
| 700 | 1 | _ | |a Huang, Yuanye |0 P:(DE-HGF)0 |b 2 |
| 700 | 1 | _ | |a Merkle, Rotraut |0 0000-0003-3811-8963 |b 3 |
| 700 | 1 | _ | |a Maier, Joachim |0 P:(DE-HGF)0 |b 4 |
| 700 | 1 | _ | |a Meulenberg, Wilhelm A. |0 P:(DE-Juel1)144923 |b 5 |
| 773 | _ | _ | |a 10.1039/D1TA05240C |g p. 10.1039.D1TA05240C |0 PERI:(DE-600)2702232-8 |p 2362-2373 |t Journal of materials chemistry / A |v 10 |y 2022 |x 2050-7496 |
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