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@ARTICLE{Qurel:902379,
      author       = {Quérel, Edouard and Seymour, Ieuan D and Cavallaro, Andrea
                      and Ma, Qianli and Tietz, Frank and Aguadero, Ainara},
      title        = {{T}he role of {N}a{SICON} surface chemistry in stabilizing
                      fast-charging {N}a metal solid-state batteries},
      journal      = {JPhys energy},
      volume       = {3},
      number       = {4},
      issn         = {2515-7655},
      address      = {Bristol},
      publisher    = {IOP Publishing},
      reportid     = {FZJ-2021-04213},
      pages        = {044007 -},
      year         = {2021},
      abstract     = {Solid-state batteries (SSBs) with alkali metal anodes hold
                      great promise as energetically dense andsafe alternatives to
                      conventional Li-ion cells. Whilst, in principle, SSBs have
                      the additionaladvantage of offering virtually unlimited
                      plating current densities, fast charges have so far onlybeen
                      achieved through sophisticated interface engineering
                      strategies. With a combination ofsurface sensitive analysis,
                      we reveal that such sophisticated engineering is not
                      necessary inNaSICON solid electrolytes
                      (Na3.4Zr2Si2.4P0.6O12) since optimised performances can be
                      achievedby simple thermal treatments that allow the
                      thermodynamic stabilization of a nanometric Na3PO4protective
                      surface layer. The optimized surface chemistry leads to
                      stabilized Na|NZSP interfaceswith exceptionally low
                      interface resistances (down to 0.1 Ωcm2 at room
                      temperature) and hightolerance to large plating current
                      densities (up to 10 mA cm−2) even for extended cycling
                      periodsof 30 min (corresponding to an areal capacity 5 mAh
                      cm−2). The created Na|NZSP interfaces showgreat stability
                      with increment of only up to 5 Ωcm2 after four months of
                      cell assembly.},
      cin          = {IEK-1},
      ddc          = {530},
      cid          = {I:(DE-Juel1)IEK-1-20101013},
      pnm          = {1223 - Batteries in Application (POF4-122)},
      pid          = {G:(DE-HGF)POF4-1223},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000717798200001},
      doi          = {10.1088/2515-7655/ac2fb3},
      url          = {https://juser.fz-juelich.de/record/902379},
}