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| Hauptseite > Publikationsdatenbank > The Impact of Lithium Tungstate on the Densification and Conductivity of Phosphate Lithium Ion Conductors > print |
| Hauptseite > Publikationsdatenbank > The Impact of Lithium Tungstate on the Densification and Conductivity of Phosphate Lithium Ion Conductors > print |
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| 245 | _ | _ | |a The Impact of Lithium Tungstate on the Densification and Conductivity of Phosphate Lithium Ion Conductors |
| 260 | _ | _ | |a Weinheim |c 2022 |b Wiley-VCH |
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| 520 | _ | _ | |a Phosphate lithium ion conductors are outstanding electrolyte materials for solid-state lithium batteries. As polycrystalline ceramics, they have to be sintered at high temperatures. Lithium tungstate Li 2 WO 4 (LWO) is reported for the first time as an effective sintering aid to reduce the sintering temperature for one of the most common solid-state lithium ion conductors, Li 1.5 Al 0.5 Ti 1.5 (PO 4 ) 3 (LATP). While densification of LATP without sintering aids requires temperatures of at least 950°C to obtain a relative density of 90%, here relative densities of 90-95% are achieved even at 775°C when 5 wt.% of LWO is added. At 800°C the LATP containing 5 - 7 wt.% LWO densifies to a relative density of 97.2%. The ionic conductivity of LWO containing LATP is generally higher than that of pure LATP sintered at the same temperature. LATP containing 7 wt.% LWO shows high ionic conductivity of 4.4 × 10 -4 S/cm after sintering at 825°C. A significant reduction in sintering temperature, an increase in density and in the ionic conductivity of LATP as well as its non toxicity render LWO a very promising sintering aid for the development of LATP-based solid state batteries. |
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| 773 | _ | _ | |a 10.1002/celc.202101366 |g p. celc.202101366 |0 PERI:(DE-600)2724978-5 |n 5 |p e202101366 |t ChemElectroChem |v 9 |y 2022 |x 2196-0216 |
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