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@ARTICLE{Jiao:902612,
author = {Jiao, Yushu and Sarwar, Sidra and Sanz, Sergio and van
Leusen, Jan and Izarova, Natalya V. and Campbell, Cameron L.
and Brechin, Euan K. and Dalgarno, Scott J. and Kögerler,
Paul},
title = {{E}xploiting complementary ligands for the construction of
square antiprismatic monometallic lanthanide {SMM}s},
journal = {Dalton transactions},
volume = {50},
number = {27},
issn = {0300-9246},
address = {London},
publisher = {Soc.},
reportid = {FZJ-2021-04407},
pages = {9648 - 9654},
year = {2021},
abstract = {The methylation of p-tert-butylcalix[4]arene in the distal
1,3-phenolic sites provides the ligand H2L =
{p-tert-butylcalix[4](OMe)2(OH)2arene} that enables
construction of heteroleptic mononuclear lanthanide
complexes. The reaction of (N(nBu)4)(acac) (Hacac =
acetylacetone), MIIICl3 and H2L under Schlenk conditions
results in the formation of a family of
(N(nBu)4)[MIIIL(acac)2] complexes where M = Y (1), Gd (2),
Tb (3) and Dy (4). The metal ions are eight-coordinate in
distorted square-antiprismatic coordination geometries,
resulting in slow relaxation of the magnetisation for the Tb
derivative.},
cin = {PGI-6},
ddc = {540},
cid = {I:(DE-Juel1)PGI-6-20110106},
pnm = {5223 - Quantum-Computer Control Systems and Cryoelectronics
(POF4-522)},
pid = {G:(DE-HGF)POF4-5223},
typ = {PUB:(DE-HGF)16},
pubmed = {34160497},
UT = {WOS:000664677600001},
doi = {10.1039/D1DT00359C},
url = {https://juser.fz-juelich.de/record/902612},
}