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@ARTICLE{Li:902945,
author = {Li, Fayong and Zhang, Qian and Klumpp, Erwin and Bol,
Roland and Nischwitz, Volker and Ge, Zhuang and Liang,
Xinqiang},
title = {{O}rganic {C}arbon {L}inkage with {S}oil {C}olloidal
{P}hosphorus at {R}egional and {F}ield {S}cales: {I}nsights
from {S}ize {F}ractionation of {F}ine {P}articles},
journal = {Environmental science $\&$ technology},
volume = {55},
number = {9},
issn = {0013-936X},
address = {Columbus, Ohio},
publisher = {American Chemical Society},
reportid = {FZJ-2021-04698},
pages = {5815 - 5825},
year = {2021},
abstract = {Nano and colloidal particles (1–1000 nm) play important
roles in phosphorus (P) migration and loss from agricultural
soils; however, little is known about their relative
distribution in arable crop soils under varying agricultural
geolandscapes at the regional scale. Surface soils (0–20
cm depth) were collected from 15 agricultural fields,
including two sites with different carbon input strategies,
in Zhejiang Province, China, and water-dispersible
nanocolloids (0.6–25 nm), fine colloids (25–160 nm), and
medium colloids (160–500 nm) were separated and analyzed
using the asymmetrical flow field flow fractionation
technique. Three levels of fine-colloidal P content
(3583–6142, 859–2612, and 514–653 μg kg–1) were
identified at the regional scale. The nanocolloidal fraction
correlated with organic carbon (Corg) and calcium (Ca), and
the fine colloidal fraction with Corg, silicon (Si),
aluminum (Al), and iron (Fe). Significant linear
relationships existed between colloidal P and Corg, Si, Al,
Fe, and Ca and for nanocolloidal P with Ca. The organic
carbon controlled colloidal P saturation, which in turn
affected the P carrier ability of colloids. Field-scale
organic carbon inputs did not change the overall
morphological trends in size fractions of water-dispersible
colloids. However, they significantly affected the peak
concentration in each of the nano-, fine-, and
medium-colloidal P fractions. Application of chemical
fertilizer with carbon-based solid manure and/or modified
biochar reduced the soil nano-, fine-, and medium-colloidal
P content by $30–40\%;$ however,the application of
chemical fertilizer with biogas slurry boosted colloidal P
formation. This study provides a deep and novel
understanding of the forms and composition of colloidal P in
agricultural soils and highlights their spatial regulation
by soil characteristics and carbon inputs.},
cin = {IBG-3},
ddc = {333.7},
cid = {I:(DE-Juel1)IBG-3-20101118},
pnm = {2173 - Agro-biogeosystems: controls, feedbacks and impact
(POF4-217)},
pid = {G:(DE-HGF)POF4-2173},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:33856195},
UT = {WOS:000648515400022},
doi = {10.1021/acs.est.0c07709},
url = {https://juser.fz-juelich.de/record/902945},
}