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000903289 1001_ $$0P:(DE-Juel1)145420$$aWei, Xian-Kui$$b0$$eCorresponding author
000903289 245__ $$aFerroelectric phase-transition frustration near a tricritical composition point
000903289 260__ $$a[London]$$bNature Publishing Group UK$$c2021
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000903289 520__ $$aPhase transition describes a mutational behavior of matter states at a critical transition temperature or external field. Despite the phase-transition orders are well sorted by classic thermodynamic theory, ambiguous situations interposed between the first- and second-order transitions were exposed one after another. Here, we report discovery of phase-transition frustration near a tricritical composition point in ferroelectric Pb(Zr1-xTix)O3. Our multi-scale transmission electron microscopy characterization reveals a number of geometrically frustrated microstructure features such as self-assembled hierarchical domain structure, degeneracy of mesoscale domain tetragonality and decoupled polarization-strain relationship. Associated with deviation from the classic mean-field theory, dielectric critical exponent anomalies and temperature dependent birefringence data unveil that the frustrated transition order stems from intricate competition of short-range polar orders and their decoupling to long-range lattice deformation. With supports from effective Hamiltonian Monte Carlo simulations, our findings point out a potentially universal mechanism to comprehend the abnormal critical phenomena occurring in phase-transition materials.
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000903289 7001_ $$00000-0003-3911-0795$$aProkhorenko, Sergei$$b1
000903289 7001_ $$0P:(DE-Juel1)186909$$aWang, Bingqing$$b2
000903289 7001_ $$00000-0002-5606-2660$$aLiu, Zenghui$$b3
000903289 7001_ $$0P:(DE-HGF)0$$aXie, Yu-Juan$$b4
000903289 7001_ $$00000-0001-8878-9760$$aNahas, Yousra$$b5
000903289 7001_ $$0P:(DE-Juel1)130736$$aJia, Chun-Lin$$b6
000903289 7001_ $$0P:(DE-Juel1)144121$$aDunin-Borkowski, Rafal E.$$b7
000903289 7001_ $$0P:(DE-Juel1)130824$$aMayer, Joachim$$b8
000903289 7001_ $$00000-0002-6181-2024$$aBellaiche, Laurent$$b9
000903289 7001_ $$0P:(DE-HGF)0$$aYe, Zuo-Guang$$b10$$eCorresponding author
000903289 773__ $$0PERI:(DE-600)2553671-0$$a10.1038/s41467-021-25543-1$$gVol. 12, no. 1, p. 5322$$n1$$p5322$$tNature Communications$$v12$$x2041-1723$$y2021
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