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| 005 | 20230310131325.0 | ||
| 024 | 7 | _ | |a 10.1038/s41467-021-25543-1 |2 doi |
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| 082 | _ | _ | |a 500 |
| 100 | 1 | _ | |a Wei, Xian-Kui |0 P:(DE-Juel1)145420 |b 0 |e Corresponding author |
| 245 | _ | _ | |a Ferroelectric phase-transition frustration near a tricritical composition point |
| 260 | _ | _ | |a [London] |c 2021 |b Nature Publishing Group UK |
| 336 | 7 | _ | |a article |2 DRIVER |
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| 520 | _ | _ | |a Phase transition describes a mutational behavior of matter states at a critical transition temperature or external field. Despite the phase-transition orders are well sorted by classic thermodynamic theory, ambiguous situations interposed between the first- and second-order transitions were exposed one after another. Here, we report discovery of phase-transition frustration near a tricritical composition point in ferroelectric Pb(Zr1-xTix)O3. Our multi-scale transmission electron microscopy characterization reveals a number of geometrically frustrated microstructure features such as self-assembled hierarchical domain structure, degeneracy of mesoscale domain tetragonality and decoupled polarization-strain relationship. Associated with deviation from the classic mean-field theory, dielectric critical exponent anomalies and temperature dependent birefringence data unveil that the frustrated transition order stems from intricate competition of short-range polar orders and their decoupling to long-range lattice deformation. With supports from effective Hamiltonian Monte Carlo simulations, our findings point out a potentially universal mechanism to comprehend the abnormal critical phenomena occurring in phase-transition materials. |
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| 700 | 1 | _ | |a Prokhorenko, Sergei |0 0000-0003-3911-0795 |b 1 |
| 700 | 1 | _ | |a Wang, Bingqing |0 P:(DE-Juel1)186909 |b 2 |
| 700 | 1 | _ | |a Liu, Zenghui |0 0000-0002-5606-2660 |b 3 |
| 700 | 1 | _ | |a Xie, Yu-Juan |0 P:(DE-HGF)0 |b 4 |
| 700 | 1 | _ | |a Nahas, Yousra |0 0000-0001-8878-9760 |b 5 |
| 700 | 1 | _ | |a Jia, Chun-Lin |0 P:(DE-Juel1)130736 |b 6 |
| 700 | 1 | _ | |a Dunin-Borkowski, Rafal E. |0 P:(DE-Juel1)144121 |b 7 |
| 700 | 1 | _ | |a Mayer, Joachim |0 P:(DE-Juel1)130824 |b 8 |
| 700 | 1 | _ | |a Bellaiche, Laurent |0 0000-0002-6181-2024 |b 9 |
| 700 | 1 | _ | |a Ye, Zuo-Guang |0 P:(DE-HGF)0 |b 10 |e Corresponding author |
| 773 | _ | _ | |a 10.1038/s41467-021-25543-1 |g Vol. 12, no. 1, p. 5322 |0 PERI:(DE-600)2553671-0 |n 1 |p 5322 |t Nature Communications |v 12 |y 2021 |x 2041-1723 |
| 856 | 4 | _ | |y OpenAccess |u https://juser.fz-juelich.de/record/903289/files/9.12.21_Wei%20et%20al.pdf |
| 856 | 4 | _ | |y OpenAccess |u https://juser.fz-juelich.de/record/903289/files/s41467-021-25543-1.pdf |
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