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@ARTICLE{Drr:903293,
author = {Dürr, S. and Zilm, S. and Geißelbrecht, M. and Müller,
Karsten and Preuster, P. and Bösmann, A. and Wasserscheid,
P.},
title = {{E}xperimental determination of the
hydrogenation/dehydrogenation - {E}quilibrium of the {LOHC}
system {H}0/{H}18-dibenzyltoluene},
journal = {International journal of hydrogen energy},
volume = {46},
number = {64},
issn = {0360-3199},
address = {New York, NY [u.a.]},
publisher = {Elsevier},
reportid = {FZJ-2021-04989},
pages = {32583 - 32594},
year = {2021},
abstract = {Liquid organic hydrogen carrier (LOHC) systems store
hydrogen through a catalystpromotedexothermal hydrogenation
reaction and release hydrogen through an
endothermalcatalytic dehydrogenation reaction. At a given
pressure and temperature theamount of releasable hydrogen
depends on the reaction equilibrium of the
hydrogenation/dehydrogenation reaction. Thus, the
equilibrium composition of a given LOHC system isone of the
key parameters for the reactor and process design of
hydrogen storage andrelease units. Currently, LOHC
equilibrium data are calculated on the basis of
calorimetricdata of selected, pure hydrogen-lean and
hydrogen-rich LOHC compounds. Yet, real reactionsystems
comprise a variety of isomers, their respective partially
hydrogenatedspecies as well as by-products formed during
multiple hydrogenation/dehydrogenationcycles. Therefore, our
study focuses on an empirical approach to describe the
temperatureand pressure dependency of the hydrogenation
equilibrium of the LOHC system H0/H18-DBT under real life
experimental conditions. Because reliable measurements of
the degree of hydrogenation (DoH) play a vital role in this
context, we describe in thiscontribution two novel methods
of DoH determination for LOHC systems based on 13C NMRand
GC-FID measurements.},
cin = {IEK-11},
ddc = {620},
cid = {I:(DE-Juel1)IEK-11-20140314},
pnm = {1232 - Power-based Fuels and Chemicals (POF4-123)},
pid = {G:(DE-HGF)POF4-1232},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000693237100008},
doi = {10.1016/j.ijhydene.2021.07.119},
url = {https://juser.fz-juelich.de/record/903293},
}