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@ARTICLE{Reissig:903294,
      author       = {Reissig, Friederike and Lange, Martin Alexander and Haneke,
                      Lukas and Placke, Tobias and Zeier, Wolfgang and Winter,
                      Martin and Schmuch, Richard and Gomez-Martin, Aurora},
      title        = {{S}ynergistic {E}ffects of {S}urface {C}oating and {B}ulk
                      {D}oping in {N}i‐{R}ich {L}ithium {N}ickel {C}obalt
                      {M}anganese {O}xide {C}athode {M}aterials for
                      {H}igh‐{E}nergy {L}ithium {I}on {B}atteries},
      journal      = {ChemSusChem},
      volume       = {15},
      number       = {4},
      issn         = {1864-5631},
      address      = {Weinheim},
      publisher    = {Wiley-VCH},
      reportid     = {FZJ-2021-04990},
      pages        = {e202102220},
      year         = {2022},
      abstract     = {Ni-rich layered oxide cathodes are promising candidates to
                      satisfy the increasing energy demand of lithium-ion
                      batteries for automotive applications. Thermal and cycling
                      stability issues originating from increasing Ni contents are
                      addressed by mitigation strategies such as elemental bulk
                      substitution (“doping”) and surface coating. Although
                      both approaches separately benefit the cycling stability,
                      there are only few reports investigating the combination of
                      two of such approaches. Herein, the combination of Zr as
                      common dopant in commercial materials with effective Li2WO4
                      and WO3 coatings was investigated with special focus on the
                      impact of different material processing conditions on
                      structural parameters and electrochemical performance in
                      nickel-cobalt-manganese (NCM) || graphite cells. Results
                      indicated that the Zr4+ dopant diffusing to the surface
                      during annealing improved the electrochemical performance
                      compared to samples without additional coatings. This work
                      emphasizes the importance to not only investigate the effect
                      of individual dopants or coatings but also the influences
                      between both.},
      cin          = {IEK-12},
      ddc          = {540},
      cid          = {I:(DE-Juel1)IEK-12-20141217},
      pnm          = {1221 - Fundamentals and Materials (POF4-122)},
      pid          = {G:(DE-HGF)POF4-1221},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {pmid:34784118},
      UT           = {WOS:000725309600001},
      doi          = {10.1002/cssc.202102220},
      url          = {https://juser.fz-juelich.de/record/903294},
}