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000903596 1001_ $$00000-0001-5830-2683$$aBrüning, D.$$b0$$eCorresponding author
000903596 245__ $$aMultiple field-induced phases in the frustrated triangular magnet Cs$_3$Fe$_2$B$_ 9$
000903596 260__ $$aWoodbury, NY$$bInst.$$c2021
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000903596 520__ $$aThe recently discovered material Cs$_3$Fe$_2$Br$_9$ contains Fe$_2$Br$_9$ bi-octahedra forming triangular layers with hexagonal stacking along the $c$ axis. In contrast to isostructural Cr-based compounds, the zero-field ground state is not a nonmagnetic S=0 singlet-dimer state. Instead, the Fe$_2$Br$_9$ bi-octahedra host semiclassical S=5/2 Fe$^{3+}$ spins with a pronounced easy-axis anisotropy along c, and interestingly, the intradimer spins are ordered ferromagnetically. The high degree of magnetic frustration due to (various) competing intradimer and interdimer couplings leads to a surprisingly rich magnetic phase diagram. The zero-field ground state is already reached via an intermediate phase, and the high-field magnetization and thermal expansion data for H∥c identify 10 different ordered phases. Among them are phases with constant magnetization of 1/3, respectively 1/2, of the saturation value, and several transitions are strongly hysteretic with pronounced length changes, reflecting strong magnetoelastic coupling.
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000903596 7001_ $$0P:(DE-HGF)0$$aFröhlich, T.$$b1
000903596 7001_ $$0P:(DE-HGF)0$$aGorkov, D.$$b2
000903596 7001_ $$0P:(DE-HGF)0$$aCísařová, I.$$b3
000903596 7001_ $$0P:(DE-HGF)0$$aSkourski, Y.$$b4
000903596 7001_ $$0P:(DE-HGF)0$$aRossi, L.$$b5
000903596 7001_ $$0P:(DE-HGF)0$$aBryant, B.$$b6
000903596 7001_ $$0P:(DE-HGF)0$$aWiedmann, S.$$b7
000903596 7001_ $$0P:(DE-Juel1)164297$$aMeven, M.$$b8
000903596 7001_ $$0P:(DE-HGF)0$$aUshakov, A.$$b9
000903596 7001_ $$00000-0002-2823-1754$$aStreltsov, S. V.$$b10
000903596 7001_ $$0P:(DE-HGF)0$$aKhomskii, D.$$b11
000903596 7001_ $$0P:(DE-Juel1)142337$$aBecker, P.$$b12
000903596 7001_ $$0P:(DE-HGF)0$$aBohatý, L.$$b13
000903596 7001_ $$0P:(DE-HGF)0$$aBraden, M.$$b14
000903596 7001_ $$0P:(DE-HGF)0$$aLorenz, T.$$b15
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