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100 1 _ |a Brüning, D.
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245 _ _ |a Multiple field-induced phases in the frustrated triangular magnet Cs$_3$Fe$_2$B$_ 9$
260 _ _ |a Woodbury, NY
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520 _ _ |a The recently discovered material Cs$_3$Fe$_2$Br$_9$ contains Fe$_2$Br$_9$ bi-octahedra forming triangular layers with hexagonal stacking along the $c$ axis. In contrast to isostructural Cr-based compounds, the zero-field ground state is not a nonmagnetic S=0 singlet-dimer state. Instead, the Fe$_2$Br$_9$ bi-octahedra host semiclassical S=5/2 Fe$^{3+}$ spins with a pronounced easy-axis anisotropy along c, and interestingly, the intradimer spins are ordered ferromagnetically. The high degree of magnetic frustration due to (various) competing intradimer and interdimer couplings leads to a surprisingly rich magnetic phase diagram. The zero-field ground state is already reached via an intermediate phase, and the high-field magnetization and thermal expansion data for H∥c identify 10 different ordered phases. Among them are phases with constant magnetization of 1/3, respectively 1/2, of the saturation value, and several transitions are strongly hysteretic with pronounced length changes, reflecting strong magnetoelastic coupling.
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700 1 _ |a Fröhlich, T.
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700 1 _ |a Gorkov, D.
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773 _ _ |a 10.1103/PhysRevB.104.064418
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