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@ARTICLE{Yu:903652,
      author       = {Yu, Shicheng and Xu, Qi and Lu, Xin and Liu, Zigeng and
                      Windmüller, Anna and Tsai, Chih-Long and Buchheit, Annika
                      and Tempel, Hermann and Kungl, Hans and Wiemhöfer,
                      Hans-Dieter and Eichel, Rüdiger-A.},
      title        = {{S}ingle-{I}on-{C}onducting “{P}olymer-in-{C}eramic”
                      {H}ybrid {E}lectrolyte with an {I}ntertwined
                      {NASICON}-{T}ype {N}anofiber {S}keleton},
      journal      = {ACS applied materials $\&$ interfaces},
      volume       = {13},
      number       = {51},
      issn         = {1944-8244},
      address      = {Washington, DC},
      publisher    = {Soc.},
      reportid     = {FZJ-2021-05301},
      pages        = {61067–61077},
      year         = {2021},
      abstract     = {The fast Li+ transportation of “polymer-in-ceramic”
                      electrolytes is highly dependent on the long-range Li+
                      migration pathways, which are determined by the structure
                      and chemistry of the electrolytes. Besides, Li dendrite
                      growth may be promoted in the soft polymer region due to the
                      inhomogeneous electric field caused by the commonly low Li+
                      transference number of the polymer. Herein, a
                      single-ion-conducting polymer electrolyte is infiltrated
                      into intertwined Li1.3Al0.3Ti1.7(PO4)3 (LATP) nanofibers to
                      construct free-standing electrolyte membranes. The composite
                      electrolyte possesses a large electrochemical window
                      exceeding 5 V, a high ionic conductivity of 0.31 mS cm–1
                      at ambient temperature, and an extraordinary Li+
                      transference number of 0.94. The hybrid electrolyte in the
                      lithium symmetric cell shows stable Li plating/stripping up
                      to 2000 h under 0.1 mA cm–2 without dendrite formation.
                      The Li|hybrid electrolyte|LiFePO4 battery exhibits enhanced
                      rate capability up to 1 C and a stable cycling performance
                      with an initial discharge capacity of 131.8 mA h g–1 and a
                      retention capacity of 122.7 mA h g–1 after 500 cycles at
                      0.5 C at ambient temperature. The improved electrochemical
                      performance is attributed to the synergistic effects of the
                      LATP nanofibers and the single-ion-conducting polymer. The
                      fibrous fast ion conductors provide continuous ion transport
                      channels, and the polymer improves the interfacial contact
                      with the electrodes and helps to suppress the Li dendrites.},
      cin          = {IEK-9 / IEK-12},
      ddc          = {600},
      cid          = {I:(DE-Juel1)IEK-9-20110218 / I:(DE-Juel1)IEK-12-20141217},
      pnm          = {1223 - Batteries in Application (POF4-122)},
      pid          = {G:(DE-HGF)POF4-1223},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {34910464},
      UT           = {WOS:000733798500001},
      doi          = {10.1021/acsami.1c17718},
      url          = {https://juser.fz-juelich.de/record/903652},
}