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@ARTICLE{Neuhaus:903677,
author = {Neuhaus, Kerstin and Schmidt, Christina and Fischer,
Liudmila and Meulenberg, Wilhelm Albert and Ran, Ke and
Mayer, Joachim and Baumann, Stefan},
title = {{M}easurement of polarization effects in dual-phase
ceria-based oxygen permeation membranes using {K}elvin probe
force microscopy},
journal = {Beilstein journal of nanotechnology},
volume = {12},
issn = {2190-4286},
address = {Frankfurt, M.},
publisher = {Beilstein-Institut zur Förderung der Chemischen
Wissenschaften},
reportid = {FZJ-2021-05326},
pages = {1380 - 1391},
year = {2021},
abstract = {In this study, a dual phase composite (CSO-FC2O) consisting
of 60 vol $\%$ Ce0.8Sm0.2O1.9 as oxygen-conductive phase and
40 vol $\%$ FeCo2O4 as electron-conductive phase was
synthesized. TEM measurements showed a relatively pure
dual-phase material with only minor amounts of a tertiary
(Sm,Ce)(Fe,Co)O3 perovskite phase and isolated residues of a
rock salt phase at the grain boundaries. The obtained
material was used as a model to demonstrate that a
combination of polarization relaxation measurements and
Kelvin probe force microscopy (KPFM)-based mapping of the
Volta potential before and after the end of polarization can
be used to determine the chemical diffusion coefficient of
the ceria component of the composite. The KPFM measurements
were performed at room temperature and show diffusion
coefficients in the range of 3 × 10−13 cm2·s−1, which
is comparable to values measured for single-phase Gd-doped
ceria thin films using the same method.},
cin = {IEK-12 / IEK-1 / ER-C-2},
ddc = {620},
cid = {I:(DE-Juel1)IEK-12-20141217 / I:(DE-Juel1)IEK-1-20101013 /
I:(DE-Juel1)ER-C-2-20170209},
pnm = {1232 - Power-based Fuels and Chemicals (POF4-123) / 1221 -
Fundamentals and Materials (POF4-122) / DFG project
387282673 - Die Rolle von Grenzflächen in mehrphasigen
Ceroxid-basierten Membranen für den Einsatz in
Membranreaktoren},
pid = {G:(DE-HGF)POF4-1232 / G:(DE-HGF)POF4-1221 /
G:(GEPRIS)387282673},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000732800000001},
doi = {10.3762/bjnano.12.102},
url = {https://juser.fz-juelich.de/record/903677},
}