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@ARTICLE{Wei:903805,
      author       = {Wei, Xian-Kui and Dunin-Borkowski, Rafal E. and Mayer,
                      Joachim},
      title        = {{S}tructural {P}hase {T}ransition and {I}n-{S}itu {E}nergy
                      {S}torage {P}athway in {N}onpolar {M}aterials: {A} {R}eview},
      journal      = {Materials},
      volume       = {14},
      number       = {24},
      issn         = {1996-1944},
      address      = {Basel},
      publisher    = {MDPI},
      reportid     = {FZJ-2021-05438},
      pages        = {7854 -},
      year         = {2021},
      abstract     = {Benefitting from exceptional energy storage performance,
                      dielectric-based capacitors are playing increasingly
                      important roles in advanced electronics and high-power
                      electrical systems. Nevertheless, a series of unresolved
                      structural puzzles represent obstacles to further improving
                      the energy storage performance. Compared with ferroelectrics
                      and linear dielectrics, antiferroelectric materials have
                      unique advantages in unlocking these puzzles due to the
                      inherent coupling of structural transitions with the energy
                      storage process. In this review, we summarize the most
                      recent studies about in-situ structural phase transitions in
                      PbZrO3-based and NaNbO3-based systems. In the context of the
                      ultrahigh energy storage density of SrTiO3-based capacitors,
                      we highlight the necessity of extending the concept of
                      antiferroelectric-to-ferroelectric (AFE-to-FE) transition to
                      broader antiferrodistortive-to-ferrodistortive (AFD-to-FD)
                      transition for materials that are simultaneously
                      ferroelastic. Combining discussion of the factors driving
                      ferroelectricity, electric-field-driven metal-to-insulator
                      transition in a (La1−xSrx)MnO3 electrode is emphasized to
                      determine the role of ionic migration in improving the
                      storage performance. We believe that this review, aiming at
                      depicting a clearer structure–property relationship, will
                      be of benefit for researchers who wish to carry out
                      cutting-edge structure and energy storage exploration},
      cin          = {ER-C-2 / ER-C-1},
      ddc          = {600},
      cid          = {I:(DE-Juel1)ER-C-2-20170209 / I:(DE-Juel1)ER-C-1-20170209},
      pnm          = {5351 - Platform for Correlative, In Situ and Operando
                      Characterization (POF4-535) / 5353 - Understanding the
                      Structural and Functional Behavior of Solid State Systems
                      (POF4-535) / DFG project 390534769 - EXC 2004: Materie und
                      Licht für Quanteninformation (ML4Q) (390534769)},
      pid          = {G:(DE-HGF)POF4-5351 / G:(DE-HGF)POF4-5353 /
                      G:(GEPRIS)390534769},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {34947446},
      UT           = {WOS:000742713100001},
      doi          = {10.3390/ma14247854},
      url          = {https://juser.fz-juelich.de/record/903805},
}