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@ARTICLE{Ovsianikov:903909,
author = {Ovsianikov, Aleksandr and Thoma, Henrik and Usmanov, Oleg
and Brown, Penelope Jane and Chatterji, Tapan and Sazonov,
Andrew and Barilo, Sergey and Peters, Lars and Hutanu,
Vladimir},
title = {{B}reaking the magnetic symmetry by reorientation
transition near 50 {K} in multiferroic magnetocaloric
{H}o{F}e{O}3},
journal = {IEEE transactions on magnetics},
volume = {58},
number = {2},
issn = {0018-9464},
address = {New York, NY},
publisher = {IEEE},
reportid = {FZJ-2021-05533},
pages = {2500105},
year = {2022},
abstract = {Using the new polarized neutron diffraction (PND) setup at
MLZ the spin reorientation transition in the magnetocaloric
orthoferrite HoFeO3 was studied at different wavelength. The
various experiments provided reproducible results
demonstrating high reliability of the used setup. We show
that during the phase transition at TSR=53 K in an external
magnetic field applied along crystal c-axis, the ordered
magnetic moment of the Fe sublattice rotates from the
crystallographic direction b to a not just in the ab plane,
but through z axis. This means that the applied field breaks
the orthorhombic symmetry allowing some magnetization
parallel to z within a short temperature region.
Interestingly, this is the same temperature region where
large magnetocaloric effect for HoFeO3 was previously
reported. A general model of the magnetic structure of
HoFeO3, unconstrained by the orthorhombic symmetry, would
allow the magnitudes and directions of the moments on each
of the 8 magnetic sublattices in the unit cell to be
independent of one-another, leading to 24 independent
magnetic parameters. PND measurements were used to determine
the absolute sign of the Dzyaloshinskii-Moriya interaction
(DMI) in the ab plane for the Fe magnetic sublattice at 65
K. DMI plays an important role in the energy balance of the
system.},
cin = {JCNS-FRM-II / JCNS-4 / JARA-FIT / MLZ},
ddc = {620},
cid = {I:(DE-Juel1)JCNS-FRM-II-20110218 /
I:(DE-Juel1)JCNS-4-20201012 / $I:(DE-82)080009_20140620$ /
I:(DE-588b)4597118-3},
pnm = {6G4 - Jülich Centre for Neutron Research (JCNS) (FZJ)
(POF4-6G4) / 632 - Materials – Quantum, Complex and
Functional Materials (POF4-632)},
pid = {G:(DE-HGF)POF4-6G4 / G:(DE-HGF)POF4-632},
experiment = {EXP:(DE-MLZ)POLI-HEIDI-20140101},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000745538100062},
doi = {10.1109/TMAG.2021.3082324},
url = {https://juser.fz-juelich.de/record/903909},
}