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@ARTICLE{Carbajo:903987,
author = {Carbajo, J. and Quintanilla, A. and Garcia-Costa, A. L. and
González-Julián, J. and Belmonte, M. and Miranzo, P. and
Osendi, M. I. and Casas, J. A.},
title = {{T}he influence of the catalyst on the {CO} formation
during catalytic wet peroxide oxidation process},
journal = {Catalysis today},
volume = {361},
issn = {0920-5861},
address = {Amsterdam},
publisher = {Elsevier},
reportid = {FZJ-2021-05557},
pages = {30 - 36},
year = {2021},
abstract = {Herein, the formation of carbon monoxide as a harmful
product upon the Catalytic Wet Peroxide Oxidation process is
studied in presence of different solid catalysts: an iron
supported activated carbon catalyst, a metal-free catalyst
based on Graphene Nanoplatelets, and $1.6 wt.\%$ Fe
containing Cr2AlC MAX phase catalyst. The CWPO performance
and the evolution of the gas effluent have been compared to
that obtained in a conventional Fenton process.Carbon
monoxide yield released was significantly lower in Catalytic
Wet Peroxide Oxidation process in relation to that obtained
in the Fenton process, where CO concentration reaches a
maximum of 6651 mg/Nm3. By contrast, in presence of
activated carbon-Fe catalyst and, notably, Graphene
Nanoplatelets and Cr2AlC MAX phase catalysts, a more
progressive phenol and aromatics intermediates oxidation
resulted in a much lower CO maximum concentration in the gas
phase at the exit of the reactor of 2454 mg/Nm3,
170 mg/Nm3 and 187 mg/Nm3, respectively.Hence, when
compared to the homogeneous Fenton oxidation, Catalytic Wet
Peroxide Oxidation process results be a more sustainable
treatment for high-loaded phenolic wastewaters by decreasing
the hazardous CO gaseous emissions avoiding this way a
secondary pollution during the oxidation process.},
cin = {IEK-1},
ddc = {540},
cid = {I:(DE-Juel1)IEK-1-20101013},
pnm = {899 - ohne Topic (POF4-899)},
pid = {G:(DE-HGF)POF4-899},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000598224600006},
doi = {10.1016/j.cattod.2019.12.020},
url = {https://juser.fz-juelich.de/record/903987},
}