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@ARTICLE{Li:903992,
      author       = {Li, Zhenwei and Zhang, Qian and Hencz, Luke and Liu, Jie
                      and Kaghazchi, Payam and Han, Jishu and Wang, Lei and Zhang,
                      Shanqing},
      title        = {{M}ultifunctional cation-vacancy-rich {Z}n{C}o2{O}4
                      polysulfide-blocking layer for ultrahigh-loading {L}i-{S}
                      battery},
      journal      = {Nano energy},
      volume       = {89},
      issn         = {2211-2855},
      address      = {Amsterdam [u.a.]},
      publisher    = {Elsevier},
      reportid     = {FZJ-2021-05562},
      pages        = {106331 -},
      year         = {2021},
      abstract     = {The major hurdle in Li-S battery commercialization is the
                      severe shuttle effect and sluggish reaction kinetics of
                      polysulfide conversion during charge-discharge cycling.
                      Herein, to overcome these barriers, we designed and
                      synthesized Zn defective Zn/Co oxide (ZDZCO) nanosheets, a
                      cation-vacancy-rich bimetallic oxide for the construction of
                      a multifunctional polysulfide-blocking layer. Both
                      theoretical and experimental studies have comprehensively
                      demonstrated that the ZDZCO shows robust binding capability
                      towards polysulfides and a high catalytic ability for fast
                      polysulfide conversion. Through a facile coating process,
                      the multifunctional ZDZCO polysulfide-blocking layer is
                      incorporated on a commercial polypropylene separator,
                      forming a composite separator. The resultant separator
                      facilitates an ultrahigh sulfur loading of 21.06 mg cm-2 and
                      an areal capacity as high as 24.25 mAh cm-2. This study
                      illuminates a promising and practical strategy to construct
                      high-performance Li-S batteries with high sulfur loading.},
      cin          = {IEK-1},
      ddc          = {660},
      cid          = {I:(DE-Juel1)IEK-1-20101013},
      pnm          = {1221 - Fundamentals and Materials (POF4-122)},
      pid          = {G:(DE-HGF)POF4-1221},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000709716200002},
      doi          = {10.1016/j.nanoen.2021.106331},
      url          = {https://juser.fz-juelich.de/record/903992},
}