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| Hauptseite > Publikationsdatenbank > Multifunctional cation-vacancy-rich ZnCo2O4 polysulfide-blocking layer for ultrahigh-loading Li-S battery > print |
| Hauptseite > Publikationsdatenbank > Multifunctional cation-vacancy-rich ZnCo2O4 polysulfide-blocking layer for ultrahigh-loading Li-S battery > print |
| 001 | 903992 | ||
| 005 | 20240708132739.0 | ||
| 024 | 7 | _ | |a 10.1016/j.nanoen.2021.106331 |2 doi |
| 024 | 7 | _ | |a 2211-2855 |2 ISSN |
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| 037 | _ | _ | |a FZJ-2021-05562 |
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| 100 | 1 | _ | |a Li, Zhenwei |0 P:(DE-HGF)0 |b 0 |
| 245 | _ | _ | |a Multifunctional cation-vacancy-rich ZnCo2O4 polysulfide-blocking layer for ultrahigh-loading Li-S battery |
| 260 | _ | _ | |a Amsterdam [u.a.] |c 2021 |b Elsevier |
| 336 | 7 | _ | |a article |2 DRIVER |
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| 336 | 7 | _ | |a Journal Article |b journal |m journal |0 PUB:(DE-HGF)16 |s 1648218600_15358 |2 PUB:(DE-HGF) |
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| 336 | 7 | _ | |a Journal Article |0 0 |2 EndNote |
| 520 | _ | _ | |a The major hurdle in Li-S battery commercialization is the severe shuttle effect and sluggish reaction kinetics of polysulfide conversion during charge-discharge cycling. Herein, to overcome these barriers, we designed and synthesized Zn defective Zn/Co oxide (ZDZCO) nanosheets, a cation-vacancy-rich bimetallic oxide for the construction of a multifunctional polysulfide-blocking layer. Both theoretical and experimental studies have comprehensively demonstrated that the ZDZCO shows robust binding capability towards polysulfides and a high catalytic ability for fast polysulfide conversion. Through a facile coating process, the multifunctional ZDZCO polysulfide-blocking layer is incorporated on a commercial polypropylene separator, forming a composite separator. The resultant separator facilitates an ultrahigh sulfur loading of 21.06 mg cm-2 and an areal capacity as high as 24.25 mAh cm-2. This study illuminates a promising and practical strategy to construct high-performance Li-S batteries with high sulfur loading. |
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| 700 | 1 | _ | |a Zhang, Qian |0 P:(DE-HGF)0 |b 1 |
| 700 | 1 | _ | |a Hencz, Luke |0 P:(DE-HGF)0 |b 2 |
| 700 | 1 | _ | |a Liu, Jie |0 P:(DE-Juel1)145655 |b 3 |e Corresponding author |
| 700 | 1 | _ | |a Kaghazchi, Payam |0 P:(DE-Juel1)174502 |b 4 |u fzj |
| 700 | 1 | _ | |a Han, Jishu |0 P:(DE-HGF)0 |b 5 |
| 700 | 1 | _ | |a Wang, Lei |0 P:(DE-Juel1)184889 |b 6 |e Corresponding author |
| 700 | 1 | _ | |a Zhang, Shanqing |0 P:(DE-HGF)0 |b 7 |e Corresponding author |
| 773 | _ | _ | |a 10.1016/j.nanoen.2021.106331 |g Vol. 89, p. 106331 - |0 PERI:(DE-600)2648700-7 |p 106331 - |t Nano energy |v 89 |y 2021 |x 2211-2855 |
| 856 | 4 | _ | |u https://juser.fz-juelich.de/record/903992/files/Multifunctional-cation-vacancy.pdf |y Published on 2021-07-10. Available in OpenAccess from 2023-07-10. |
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