000904102 001__ 904102
000904102 005__ 20240712084513.0
000904102 0247_ $$2doi$$a10.1021/acsami.0c20958
000904102 0247_ $$2ISSN$$a1944-8244
000904102 0247_ $$2ISSN$$a1944-8252
000904102 0247_ $$2Handle$$a2128/30269
000904102 0247_ $$2altmetric$$aaltmetric:99208646
000904102 0247_ $$2pmid$$apmid:33513304
000904102 0247_ $$2WOS$$aWOS:000619638400095
000904102 037__ $$aFZJ-2021-05672
000904102 082__ $$a600
000904102 1001_ $$0P:(DE-HGF)0$$aGünzler, Antonio$$b0
000904102 245__ $$aShaping Perovskites: In Situ Crystallization Mechanism of Rapid Thermally Annealed, Prepatterned Perovskite Films
000904102 260__ $$aWashington, DC$$bSoc.$$c2021
000904102 3367_ $$2DRIVER$$aarticle
000904102 3367_ $$2DataCite$$aOutput Types/Journal article
000904102 3367_ $$0PUB:(DE-HGF)16$$2PUB:(DE-HGF)$$aJournal Article$$bjournal$$mjournal$$s1642413692_30509
000904102 3367_ $$2BibTeX$$aARTICLE
000904102 3367_ $$2ORCID$$aJOURNAL_ARTICLE
000904102 3367_ $$00$$2EndNote$$aJournal Article
000904102 520__ $$aUnderstanding and controlling the crystallization of organic–inorganic perovskite materials is important for their function in optoelectronic applications. This control is particularly delicate in scalable single-step thermal annealing methods. In this work, the crystallization mechanisms of flash infrared-annealed perovskite films, grown on substrates with lithographically patterned Au nucleation seeds, are investigated. The patterning enables the in situ observation to study the crystallization kinetics and the precise control of the perovskite nucleation and domain growth, while retaining the characteristic polycrystalline micromorphology with larger crystallites at the boundaries of the crystal domains, as shown by electron backscattering diffraction. Time-resolved photoluminescence measurements reveal longer charge carrier lifetimes in regions with large crystallites on the domain boundaries, relative to the domain interior. By increasing the nucleation site density, the proportion of larger crystallites is increased. This study shows that the combination of rapid thermal annealing with nucleation control is a promising approach to improve perovskite crystallinity and thereby ultimately the performance of optoelectronic devices.
000904102 536__ $$0G:(DE-HGF)POF4-1212$$a1212 - Materials and Interfaces (POF4-121)$$cPOF4-121$$fPOF IV$$x0
000904102 588__ $$aDataset connected to CrossRef, Journals: juser.fz-juelich.de
000904102 7001_ $$00000-0002-8964-9660$$aBermúdez-Ureña, Esteban$$b1
000904102 7001_ $$00000-0002-0559-4085$$aMuscarella, Loreta A.$$b2
000904102 7001_ $$0P:(DE-HGF)0$$aOchoa, Mario$$b3
000904102 7001_ $$0P:(DE-HGF)0$$aOchoa-Martínez, Efraín$$b4
000904102 7001_ $$0P:(DE-HGF)0$$aEhrler, Bruno$$b5
000904102 7001_ $$0P:(DE-Juel1)180101$$aSaliba, Michael$$b6
000904102 7001_ $$00000-0001-5936-339X$$aSteiner, Ullrich$$b7$$eCorresponding author
000904102 773__ $$0PERI:(DE-600)2467494-1$$a10.1021/acsami.0c20958$$gVol. 13, no. 5, p. 6854 - 6863$$n5$$p6854 - 6863$$tACS applied materials & interfaces$$v13$$x1944-8244$$y2021
000904102 8564_ $$uhttps://juser.fz-juelich.de/record/904102/files/acsami.0c20958.pdf$$yOpenAccess
000904102 909CO $$ooai:juser.fz-juelich.de:904102$$pdnbdelivery$$pdriver$$pVDB$$popen_access$$popenaire
000904102 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)180101$$aForschungszentrum Jülich$$b6$$kFZJ
000904102 9131_ $$0G:(DE-HGF)POF4-121$$1G:(DE-HGF)POF4-120$$2G:(DE-HGF)POF4-100$$3G:(DE-HGF)POF4$$4G:(DE-HGF)POF$$9G:(DE-HGF)POF4-1212$$aDE-HGF$$bForschungsbereich Energie$$lMaterialien und Technologien für die Energiewende (MTET)$$vPhotovoltaik und Windenergie$$x0
000904102 9141_ $$y2021
000904102 915__ $$0StatID:(DE-HGF)0200$$2StatID$$aDBCoverage$$bSCOPUS$$d2021-01-30
000904102 915__ $$0StatID:(DE-HGF)0300$$2StatID$$aDBCoverage$$bMedline$$d2021-01-30
000904102 915__ $$0StatID:(DE-HGF)1160$$2StatID$$aDBCoverage$$bCurrent Contents - Engineering, Computing and Technology$$d2021-01-30
000904102 915__ $$0LIC:(DE-HGF)CCBYNCND4$$2HGFVOC$$aCreative Commons Attribution-NonCommercial-NoDerivs CC BY-NC-ND 4.0
000904102 915__ $$0StatID:(DE-HGF)1150$$2StatID$$aDBCoverage$$bCurrent Contents - Physical, Chemical and Earth Sciences$$d2021-01-30
000904102 915__ $$0StatID:(DE-HGF)9905$$2StatID$$aIF >= 5$$bACS APPL MATER INTER : 2019$$d2021-01-30
000904102 915__ $$0StatID:(DE-HGF)0113$$2StatID$$aWoS$$bScience Citation Index Expanded$$d2021-01-30
000904102 915__ $$0StatID:(DE-HGF)0150$$2StatID$$aDBCoverage$$bWeb of Science Core Collection$$d2021-01-30
000904102 915__ $$0StatID:(DE-HGF)0510$$2StatID$$aOpenAccess
000904102 915__ $$0StatID:(DE-HGF)0100$$2StatID$$aJCR$$bACS APPL MATER INTER : 2019$$d2021-01-30
000904102 915__ $$0StatID:(DE-HGF)0160$$2StatID$$aDBCoverage$$bEssential Science Indicators$$d2021-01-30
000904102 915__ $$0StatID:(DE-HGF)0199$$2StatID$$aDBCoverage$$bClarivate Analytics Master Journal List$$d2021-01-30
000904102 920__ $$lyes
000904102 9201_ $$0I:(DE-Juel1)IEK-5-20101013$$kIEK-5$$lPhotovoltaik$$x0
000904102 9801_ $$aFullTexts
000904102 980__ $$ajournal
000904102 980__ $$aVDB
000904102 980__ $$aUNRESTRICTED
000904102 980__ $$aI:(DE-Juel1)IEK-5-20101013
000904102 981__ $$aI:(DE-Juel1)IMD-3-20101013