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000904107 1001_ $$0P:(DE-HGF)0$$aMohammadi, Mahdi$$b0
000904107 245__ $$aEncapsulation Strategies for Highly Stable Perovskite Solar Cells under Severe Stress Testing: Damp Heat, Freezing, and Outdoor Illumination Conditions
000904107 260__ $$aWashington, DC$$bSoc.$$c2021
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000904107 520__ $$aA key direction toward managing extrinsic instabilities in perovskite solar cells (PSCs) is encapsulation. Thus, a suitable sealing layer is required for an efficient device encapsulation, preventing moisture and oxygen ingression into the perovskite layer. In this work, a solution-based, low-cost, and commercially available bilayer structure of poly(methyl methacrylate)/styrene-butadiene (PMMA/SB) is investigated for PSCs encapsulation. Encapsulated devices retained 80% of the initial power conversion efficiency (PCE) at 85 °C temperature and 85% relative humidity after 100 h, while reference devices without SB (only PMMA) suffer from rapid and intense degradation after only 2 h, under the same condition. In addition, encapsulated devices retained 95% of the initial PCE under −15 °C freezing temperature after 6 h and retained ∼80% of the initial PCE after immersion in HCl (37%) for 90 min. Moreover, applying an additional aluminum metal sheet on the PMMA/SB protective bilayer leads to the improvement of device stability up to 500 h under outdoor illumination, retaining almost 90% of the initial PCE. Considering the urge to develop reliable, scalable, and simple encapsulation for future large-area PSCs, this work establishes solution-based bilayer encapsulation, which is applicable for flexible solar modules as well as other optoelectronic devices such as light-emitting devices and photodetectors.
000904107 536__ $$0G:(DE-HGF)POF4-1214$$a1214 - Modules, stability, performance and specific applications (POF4-121)$$cPOF4-121$$fPOF IV$$x0
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000904107 7001_ $$0P:(DE-HGF)0$$aGholipour, Somayeh$$b1
000904107 7001_ $$0P:(DE-HGF)0$$aMalekshahi Byranvand, Mahdi$$b2
000904107 7001_ $$00000-0002-7583-7687$$aAbdi, Yaser$$b3
000904107 7001_ $$00000-0001-6815-2041$$aTaghavinia, Nima$$b4
000904107 7001_ $$0P:(DE-Juel1)180101$$aSaliba, Michael$$b5$$eCorresponding author
000904107 773__ $$0PERI:(DE-600)2467494-1$$a10.1021/acsami.1c11628$$gVol. 13, no. 38, p. 45455 - 45464$$n38$$p45455 - 45464$$tACS applied materials & interfaces$$v13$$x1944-8244$$y2021
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