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@ARTICLE{Stockwell:904155,
      author       = {Stockwell, Chelsea E. and Coggon, Matthew M. and Gkatzelis,
                      Georgios and Ortega, John and McDonald, Brian C. and
                      Peischl, Jeff and Aikin, Kenneth and Gilman, Jessica B. and
                      Trainer, Michael and Warneke, Carsten},
      title        = {{V}olatile organic compound emissions from solvent- and
                      water-borne coatings – compositional differences and
                      tracer compound identifications},
      journal      = {Atmospheric chemistry and physics},
      volume       = {21},
      number       = {8},
      issn         = {1680-7316},
      address      = {Katlenburg-Lindau},
      publisher    = {EGU},
      reportid     = {FZJ-2021-05725},
      pages        = {6005 - 6022},
      year         = {2021},
      abstract     = {The emissions of volatile organic compounds (VOCs) from
                      volatile chemical products (VCPs) – specifically personal
                      care products, cleaning agents, coatings, adhesives, and
                      pesticides – are emerging as the largest source of
                      petroleum-derived organic carbon in US cities. Previous work
                      has shown that the ambient concentration of markers for most
                      VCP categories correlates strongly with population density,
                      except for VOCs predominantly originating from solvent- and
                      water-borne coatings (e.g., parachlorobenzotrifluoride
                      (PCBTF) and Texanol®, respectively). Instead, these
                      enhancements were dominated by distinct emission events
                      likely driven by industrial usage patterns, such as
                      construction activity. In this work, the headspace of a
                      variety of coating products was analyzed using a
                      proton-transfer-reaction time-of-flight mass spectrometer
                      (PTR-ToF-MS) and a gas chromatography (GC) preseparation
                      front end to identify composition differences for various
                      coating types (e.g., paints, primers, sealers, and stains).
                      Evaporation experiments of several products showed high
                      initial VOC emission rates, and for the length of these
                      experiments, the majority of the VOC mass was emitted during
                      the first few hours following application. The percentage of
                      mass emitted as measured VOCs $(<1 \%$ to $83 \%)$
                      mirrored the VOC content reported by the manufacturer (<5 to
                      550 g L−1). Ambient and laboratory measurements, usage
                      trends, and ingredients compiled from architectural coatings
                      surveys show that both PCBTF and Texanol account for
                      $∼10 \%$ of the total VOC ingredient sales and,
                      therefore, can be useful tracers for solvent- and
                      water-borne coatings.},
      cin          = {IEK-8},
      ddc          = {550},
      cid          = {I:(DE-Juel1)IEK-8-20101013},
      pnm          = {2111 - Air Quality (POF4-211)},
      pid          = {G:(DE-HGF)POF4-2111},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000643555400003},
      doi          = {10.5194/acp-21-6005-2021},
      url          = {https://juser.fz-juelich.de/record/904155},
}