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000904167 0247_ $$2doi$$a10.1021/acsaem.1c02278
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000904167 1001_ $$0P:(DE-Juel1)173744$$aJiang, Ming$$b0$$ufzj
000904167 245__ $$aFormation of a Stable Solid-Electrolyte Interphase at Metallic Lithium Anodes Induced by LiNbO 3 Protective Layers
000904167 260__ $$aWashington, DC$$bACS Publications$$c2021
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000904167 520__ $$aThe stability of solid-electrolyte interphase (SEI) surface films at Li-metal anodes is crucial for the safe and durable operation of lithium-metal batteries (LMBs). By combining Li-metal anodes with high-performance Ni-rich transition-metal oxide cathodes, LMBs can meet the goal of a high specific energy density of more than 500 Wh kg–1. However, Li-metal anodes suffer from serious problems, especially the nonuniform lithium deposition and uncontrollable SEI formation. In this work, Li-metal anodes were protected by thin-film LiNbO3 coatings. Full cells composed of protected Li-metal anodes and LiNi0.6Co0.2Mn0.2O2 cathodes were examined electrochemically and by physical characterization methods. Postmortem analyses of pristine and prolonged cycled Li-metal anodes were performed. The results revealed the formation of more stable SEI films at the protected Li-metal anodes in comparison to unprotected electrodes. Consequently, the LiNbO3 layers improved the cycle-life performance of Li-metal anodes in LMBs. Furthermore, X-ray photoelectron spectroscopy (XPS) analyses showed that the reduction of metallic ions stemming from the Ni-rich cathodes was also inhibited by the protective LiNbO3 layers, thereby further controlling the degradation of Li-metal anodes.
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000904167 7001_ $$0P:(DE-Juel1)176830$$aZhang, Qian$$b1$$ufzj
000904167 7001_ $$0P:(DE-Juel1)173719$$aDanilov, Dmitri$$b2$$ufzj
000904167 7001_ $$0P:(DE-Juel1)156123$$aEichel, Rüdiger-A.$$b3
000904167 7001_ $$0P:(DE-Juel1)165918$$aNotten, Peter H. L.$$b4$$eCorresponding author$$ufzj
000904167 773__ $$0PERI:(DE-600)2916551-9$$a10.1021/acsaem.1c02278$$gVol. 4, no. 9, p. 10333 - 10343$$n9$$p10333 - 10343$$tACS applied energy materials$$v4$$x2574-0962$$y2021
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000904167 9101_ $$0I:(DE-HGF)0$$6P:(DE-Juel1)165918$$a University of Technology Sydney$$b4
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000904167 9141_ $$y2021
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